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Leigang Li, Pengtang Wang, Qi Shao, Xiaoqing Huang
Proton exchange membrane (PEM) water electrolyzers hold great significance for renewable energy storage and conversion. The acidic oxygen evolution reaction (OER) is one of the main roadblocks that hinder the practical application of PEM water electrolyzers. Highly active, cost-effective, and durable electrocatalysts are indispensable for lowering the high kinetic barrier of OER to achieve boosted reaction kinetics. To date, a wide spectrum of advanced electrocatalysts has been designed and synthesized for enhanced acidic OER performance, though Ir and Ru based nanostructures still represent the state-of-the-art catalysts. In this Progress Report, recent research progress in advanced electrocatalysts for improved acidic OER performance is summarized. First, fundamental understanding about acidic OER including reaction mechanisms and atomic understanding to acidic OER for rational design of efficient electrocatalysts are discussed. Thereafter, an overview of the progress in the design and synthesis of advanced acidic OER electrocatalysts is provided in terms of catalyst category, i.e., metallic nanostructures (Ir and Ru based), precious metal oxides, nonprecious metal oxides, and carbon based nanomaterials. Finally, perspectives to the future development of acidic OER are provided from the aspects of reaction mechanism investigation and more efficient electrocatalyst design.
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Li, L., Wang, P., Shao, Q., & Huang, X. (2021). Recent Progress in Advanced Electrocatalyst Design for Acidic Oxygen Evolution Reaction. Advanced Materials, 33(50), e2004243. https://doi.org/10.1002/adma.202004243
Li, Leigang, et al. "Recent Progress in Advanced Electrocatalyst Design for Acidic Oxygen Evolution Reaction." Advanced Materials, vol. 33, no. 50, 2021, pp. e2004243, https://doi.org/10.1002/adma.202004243.
Li, Leigang, Pengtang Wang, Qi Shao, and Xiaoqing Huang. "Recent Progress in Advanced Electrocatalyst Design for Acidic Oxygen Evolution Reaction." Advanced Materials 33, no. 50 (2021): e2004243. https://doi.org/10.1002/adma.202004243.
Li L., Wang P., Shao Q. [и др.] Recent Progress in Advanced Electrocatalyst Design for Acidic Oxygen Evolution Reaction // Advanced Materials. — 2021. — Vol. 33, № 50. — P. e2004243. — URL: https://doi.org/10.1002/adma.202004243
@article{li2021recent,
title = {{Recent Progress in Advanced Electrocatalyst Design for Acidic Oxygen Evolution Reaction}},
author = {Leigang Li and Pengtang Wang and Qi Shao and Xiaoqing Huang},
journal = {Advanced Materials},
year = {2021},
volume = {33},
number = {50},
pages = {e2004243},
doi = {10.1002/adma.202004243},
url = {https://doi.org/10.1002/adma.202004243}
}TY - JOUR AU - Li, Leigang AU - Wang, Pengtang AU - Shao, Qi AU - Huang, Xiaoqing TI - Recent Progress in Advanced Electrocatalyst Design for Acidic Oxygen Evolution Reaction JO - Advanced Materials VL - 33 IS - 50 SP - e2004243 PY - 2021 DA - 2021/03/21 DO - 10.1002/adma.202004243 UR - https://doi.org/10.1002/adma.202004243 ER -
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