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Ben Zhang, Yijuan Zheng, Tian Ma, Chengdong Yang, Yifei Peng, Z. C. Zhou, Mi Zhou, Shuang Li, Yinghan Wang, Chong Cheng
Electrochemical water splitting has attracted significant attention as a key pathway for the development of renewable energy systems. Fabricating efficient electrocatalysts for these processes is intensely desired to reduce their overpotentials and facilitate practical applications. Recently, metal-organic framework (MOF) nanoarchitectures featuring ultrahigh surface areas, tunable nanostructures, and excellent porosities have emerged as promising materials for the development of highly active catalysts for electrochemical water splitting. Herein, the most pivotal advances in recent research on engineering MOF nanoarchitectures for efficient electrochemical water splitting are presented. First, the design of catalytic centers for MOF-based/derived electrocatalysts is summarized and compared from the aspects of chemical composition optimization and structural functionalization at the atomic and molecular levels. Subsequently, the fast-growing breakthroughs in catalytic activities, identification of highly active sites, and fundamental mechanisms are thoroughly discussed. Finally, a comprehensive commentary on the current primary challenges and future perspectives in water splitting and its commercialization for hydrogen production is provided. Hereby, new insights into the synthetic principles and electrocatalysis for designing MOF nanoarchitectures for the practical utilization of water splitting are offered, thus further promoting their future prosperity for a wide range of applications.
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Zhang, B., Zheng, Y., Ma, T., Yang, C., Peng, Y., Zhou, Z. C., Zhou, M., Li, S., Wang, Y., & Cheng, C. (2021). Designing MOF Nanoarchitectures for Electrochemical Water Splitting. Advanced Materials, 33(17), e2006042. https://doi.org/10.1002/adma.202006042
Zhang, Ben, et al. "Designing MOF Nanoarchitectures for Electrochemical Water Splitting." Advanced Materials, vol. 33, no. 17, 2021, pp. e2006042, https://doi.org/10.1002/adma.202006042.
Zhang, Ben, Yijuan Zheng, Tian Ma, Chengdong Yang, Yifei Peng, Z. C. Zhou, Mi Zhou, Shuang Li, Yinghan Wang, and Chong Cheng. "Designing MOF Nanoarchitectures for Electrochemical Water Splitting." Advanced Materials 33, no. 17 (2021): e2006042. https://doi.org/10.1002/adma.202006042.
Zhang B., Zheng Y., Ma T. [и др.] Designing MOF Nanoarchitectures for Electrochemical Water Splitting // Advanced Materials. — 2021. — Vol. 33, № 17. — P. e2006042. — URL: https://doi.org/10.1002/adma.202006042
@article{zhang2021designing,
title = {{Designing MOF Nanoarchitectures for Electrochemical Water Splitting}},
author = {Ben Zhang and Yijuan Zheng and Tian Ma and Chengdong Yang and Yifei Peng and Z. C. Zhou and Mi Zhou and Shuang Li and Yinghan Wang and Chong Cheng},
journal = {Advanced Materials},
year = {2021},
volume = {33},
number = {17},
pages = {e2006042},
doi = {10.1002/adma.202006042},
url = {https://doi.org/10.1002/adma.202006042}
}TY - JOUR AU - Zhang, Ben AU - Zheng, Yijuan AU - Ma, Tian AU - Yang, Chengdong AU - Peng, Yifei AU - Zhou, Z. C. AU - Zhou, Mi AU - Li, Shuang AU - Wang, Yinghan AU - Cheng, Chong TI - Designing MOF Nanoarchitectures for Electrochemical Water Splitting JO - Advanced Materials VL - 33 IS - 17 SP - e2006042 PY - 2021 DA - 2021/03/22 DO - 10.1002/adma.202006042 UR - https://doi.org/10.1002/adma.202006042 ER -
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