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Li An, Chao Wei, Min Lu, Hanwen Liu, Yubo Chen, Günther G. Scherer, Adrian C. Fisher, Pinxian Xi, Zhichuan Jason Xu, Chun‐Hua Yan
The proton exchange membrane (PEM) water electrolysis is one of the most promising hydrogen production techniques. The oxygen evolution reaction (OER) occurring at the anode dominates the overall efficiency. Developing active and robust electrocatalysts for OER in acid is a longstanding challenge for PEM water electrolyzers. Most catalysts show unsatisfied stability under strong acidic and oxidative conditions. Such a stability challenge also leads to difficulties for a better understanding of mechanisms. This review aims to provide the current progress on understanding of OER mechanisms in acid, analyze the promising strategies to enhance both activity and stability, and summarize the state-of-the-art catalysts for OER in acid. First, the prevailing OER mechanisms are reviewed to establish the physicochemical structure-activity relationships for guiding the design of highly efficient OER electrocatalysts in acid with stable performance. The reported approaches to improve the activity, from macroview to microview, are then discussed. To analyze the problem of instability, the key factors affecting catalyst stability are summarized and the surface reconstruction is discussed. Various noble-metal-based OER catalysts and the current progress of non-noble-metal-based catalysts are reviewed. Finally, the challenges and perspectives for the development of active and robust OER catalysts in acid are discussed.
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An, L., Wei, C., Lu, M., Liu, H., Chen, Y., Scherer, G. G., Fisher, A. C., Xi, P., Xu, Z. J., & Yan, C. (2021). Recent Development of Oxygen Evolution Electrocatalysts in Acidic Environment. Advanced Materials, 33(20), e2006328. https://doi.org/10.1002/adma.202006328
An, Li, et al. "Recent Development of Oxygen Evolution Electrocatalysts in Acidic Environment." Advanced Materials, vol. 33, no. 20, 2021, pp. e2006328, https://doi.org/10.1002/adma.202006328.
An, Li, Chao Wei, Min Lu, Hanwen Liu, Yubo Chen, Günther G. Scherer, Adrian C. Fisher, Pinxian Xi, Zhichuan Jason Xu, and Chun‐Hua Yan. "Recent Development of Oxygen Evolution Electrocatalysts in Acidic Environment." Advanced Materials 33, no. 20 (2021): e2006328. https://doi.org/10.1002/adma.202006328.
An L., Wei C., Lu M. [и др.] Recent Development of Oxygen Evolution Electrocatalysts in Acidic Environment // Advanced Materials. — 2021. — Vol. 33, № 20. — P. e2006328. — URL: https://doi.org/10.1002/adma.202006328
@article{an2021recent,
title = {{Recent Development of Oxygen Evolution Electrocatalysts in Acidic Environment}},
author = {Li An and Chao Wei and Min Lu and Hanwen Liu and Yubo Chen and Günther G. Scherer and Adrian C. Fisher and Pinxian Xi and Zhichuan Jason Xu and Chun‐Hua Yan},
journal = {Advanced Materials},
year = {2021},
volume = {33},
number = {20},
pages = {e2006328},
doi = {10.1002/adma.202006328},
url = {https://doi.org/10.1002/adma.202006328}
}TY - JOUR AU - An, Li AU - Wei, Chao AU - Lu, Min AU - Liu, Hanwen AU - Chen, Yubo AU - Scherer, Günther G. AU - Fisher, Adrian C. AU - Xi, Pinxian AU - Xu, Zhichuan Jason AU - Yan, Chun‐Hua TI - Recent Development of Oxygen Evolution Electrocatalysts in Acidic Environment JO - Advanced Materials VL - 33 IS - 20 SP - e2006328 PY - 2021 DA - 2021/03/25 DO - 10.1002/adma.202006328 UR - https://doi.org/10.1002/adma.202006328 ER -
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