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Xianjie Chen, Jun Wang, Yongqiang Chai, Zijian Zhang, Yongfa Zhu
A graphitic carbon nitride/rGO/perylene diimide polymer (g‐C 3 N 4 /rGO/PDIP) Z‐scheme heterojunction is successfully constructed to realize high‐flux charge transfer and efficient photocatalytic overall water splitting. A giant internal electric field in the Z‐scheme junction is built, enabling the charge separation efficiency to be enhanced dramatically by 8.5 times. Thus, g‐C 3 N 4 /rGO/PDIP presents an efficient and stable photocatalytic overall water splitting activity with H 2 and O 2 evolution rate of 15.80 and 7.80 µmol h −1 , respectively, ≈12.1 times higher than g‐C 3 N 4 nanosheets. Meanwhile, a notable quantum efficiency of 4.94% at 420 nm and solar‐to‐hydrogen energy‐conversion efficiency of 0.30% are achieved, prominently surpassing many reported g‐C 3 N 4 ‐based photocatalysts. Briefly, this work throws light on enhancing the internal electric field by interface control to dramatically improve the photocatalytic performance.
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Chen, X., Wang, J., Chai, Y., Zhang, Z., & Zhu, Y. (2021). Efficient Photocatalytic Overall Water Splitting Induced by the Giant Internal Electric Field of a g‐C 3 N 4 /rGO/PDIP Z‐Scheme Heterojunction. Advanced Materials, 33(7), e2007479. https://doi.org/10.1002/adma.202007479
Chen, Xianjie, et al. "Efficient Photocatalytic Overall Water Splitting Induced by the Giant Internal Electric Field of a g‐C 3 N 4 /rGO/PDIP Z‐Scheme Heterojunction." Advanced Materials, vol. 33, no. 7, 2021, pp. e2007479, https://doi.org/10.1002/adma.202007479.
Chen, Xianjie, Jun Wang, Yongqiang Chai, Zijian Zhang, and Yongfa Zhu. "Efficient Photocatalytic Overall Water Splitting Induced by the Giant Internal Electric Field of a g‐C 3 N 4 /rGO/PDIP Z‐Scheme Heterojunction." Advanced Materials 33, no. 7 (2021): e2007479. https://doi.org/10.1002/adma.202007479.
Chen X., Wang J., Chai Y. [и др.] Efficient Photocatalytic Overall Water Splitting Induced by the Giant Internal Electric Field of a g‐C 3 N 4 /rGO/PDIP Z‐Scheme Heterojunction // Advanced Materials. — 2021. — Vol. 33, № 7. — P. e2007479. — URL: https://doi.org/10.1002/adma.202007479
@article{chen2021efficient,
title = {{Efficient Photocatalytic Overall Water Splitting Induced by the Giant Internal Electric Field of a g‐C 3 N 4 /rGO/PDIP Z‐Scheme Heterojunction}},
author = {Xianjie Chen and Jun Wang and Yongqiang Chai and Zijian Zhang and Yongfa Zhu},
journal = {Advanced Materials},
year = {2021},
volume = {33},
number = {7},
pages = {e2007479},
doi = {10.1002/adma.202007479},
url = {https://doi.org/10.1002/adma.202007479}
}TY - JOUR AU - Chen, Xianjie AU - Wang, Jun AU - Chai, Yongqiang AU - Zhang, Zijian AU - Zhu, Yongfa TI - Efficient Photocatalytic Overall Water Splitting Induced by the Giant Internal Electric Field of a g‐C 3 N 4 /rGO/PDIP Z‐Scheme Heterojunction JO - Advanced Materials VL - 33 IS - 7 SP - e2007479 PY - 2021 DA - 2021/01/14 DO - 10.1002/adma.202007479 UR - https://doi.org/10.1002/adma.202007479 ER -
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