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Chang Cheng, Bowen He, Jiajie Fan, Bei Cheng, Shaowen Cao, Jiaguo Yu
Inspired by natural photosynthesis, constructing inorganic/organic heterojunctions is regarded as an effective strategy to design high‐efficiency photocatalysts. Herein, a step (S)‐scheme heterojunction photocatalyst is prepared by in situ growth of an inorganic semiconductor firmly on an organic semiconductor. A new pyrene‐based conjugated polymer, pyrene‐ alt ‐triphenylamine (PT), is synthesized via the typical Suzuki–Miyaura reactions, and then employed as a substrate to anchor CdS nanocrystals. The optimized CdS/PT composite, coupling 2 wt% PT with CdS, exhibits a robust H 2 evolution rate of 9.28 mmol h −1 g −1 with continuous release of H 2 bubbles, as well as a high apparent quantum efficiency of 24.3%, which is ≈8 times that of pure CdS. The S‐scheme charge transfer mechanism between PT and CdS, is systematically demonstrated by photoirradiated Kelvin probe measurement and in situ irradiated X‐ray photoelectron spectroscopy analyses. This work provides a protocol for preparing specific S‐scheme heterojunction photocatalysts on the basis of inorganic/organic coupling.
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Cheng, C., He, B., Fan, J., Cheng, B., Cao, S., & Yu, J. (2021). An Inorganic/Organic S‐Scheme Heterojunction H 2 ‐Production Photocatalyst and its Charge Transfer Mechanism. Advanced Materials, 33(22), e2100317. https://doi.org/10.1002/adma.202100317
Cheng, Chang, et al. "An Inorganic/Organic S‐Scheme Heterojunction H 2 ‐Production Photocatalyst and its Charge Transfer Mechanism." Advanced Materials, vol. 33, no. 22, 2021, pp. e2100317, https://doi.org/10.1002/adma.202100317.
Cheng, Chang, Bowen He, Jiajie Fan, Bei Cheng, Shaowen Cao, and Jiaguo Yu. "An Inorganic/Organic S‐Scheme Heterojunction H 2 ‐Production Photocatalyst and its Charge Transfer Mechanism." Advanced Materials 33, no. 22 (2021): e2100317. https://doi.org/10.1002/adma.202100317.
Cheng C., He B., Fan J. [и др.] An Inorganic/Organic S‐Scheme Heterojunction H 2 ‐Production Photocatalyst and its Charge Transfer Mechanism // Advanced Materials. — 2021. — Vol. 33, № 22. — P. e2100317. — URL: https://doi.org/10.1002/adma.202100317
@article{cheng2021inorganicorganic,
title = {{An Inorganic/Organic S‐Scheme Heterojunction H 2 ‐Production Photocatalyst and its Charge Transfer Mechanism}},
author = {Chang Cheng and Bowen He and Jiajie Fan and Bei Cheng and Shaowen Cao and Jiaguo Yu},
journal = {Advanced Materials},
year = {2021},
volume = {33},
number = {22},
pages = {e2100317},
doi = {10.1002/adma.202100317},
url = {https://doi.org/10.1002/adma.202100317}
}TY - JOUR AU - Cheng, Chang AU - He, Bowen AU - Fan, Jiajie AU - Cheng, Bei AU - Cao, Shaowen AU - Yu, Jiaguo TI - An Inorganic/Organic S‐Scheme Heterojunction H 2 ‐Production Photocatalyst and its Charge Transfer Mechanism JO - Advanced Materials VL - 33 IS - 22 SP - e2100317 PY - 2021 DA - 2021/04/26 DO - 10.1002/adma.202100317 UR - https://doi.org/10.1002/adma.202100317 ER -
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