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Peng Zhou, Xingshuai Lv, Shasha Tao, Jingcheng Wu, Hongfang Wang, Xiaoxiao Wei, Tehua Wang, Bo Zhou, Yuxuan Lu, Thomas Frauenheim and 3 more
Electrocatalytic oxidation of 5‐hydroxymethylfurfural (HMF) provides an efficient way to obtain high‐value‐added biomass‐derived chemicals. Compared with other transition metal oxides, CuO exhibits poor oxygen evolution reaction performance, leading to high Faraday efficiency for HMF oxidation. However, the weak adsorption and activation ability of CuO to OH − species restricts its further development. Herein, the CuO–PdO heterogeneous interface is successfully constructed, resulting in an advanced onset‐potential of the HMF oxidation reaction (HMFOR), a higher current density than CuO. The results of open‐circuit potential, in situ infrared spectroscopy, and theoretical calculations indicate that the introduction of PdO enhances the adsorption capacity of the organic molecule. Meanwhile, the CuO–PdO heterogeneous interface promotes the adsorption and activation of OH − species, as demonstrated by zeta potential and electrochemical measurements. This work elucidates the adsorption enhancement mechanism of heterogeneous interfaces and provides constructive guidance for designing efficient multicomponent electrocatalysts in organic electrocatalytic reactions.
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Zhou, P., Lv, X., Tao, S., Wu, J., Wang, H., Wei, X., Wang, T., Zhou, B., Lu, Y., Frauenheim, T., Fu, X., Wang, S., & Zou, Y. (2022). Heterogeneous‐Interface‐Enhanced Adsorption of Organic and Hydroxyl for Biomass Electrooxidation. Advanced Materials, 34(42), e2204089. https://doi.org/10.1002/adma.202204089
Zhou, Peng, et al. "Heterogeneous‐Interface‐Enhanced Adsorption of Organic and Hydroxyl for Biomass Electrooxidation." Advanced Materials, vol. 34, no. 42, 2022, pp. e2204089, https://doi.org/10.1002/adma.202204089.
Zhou, Peng, Xingshuai Lv, Shasha Tao, Jingcheng Wu, Hongfang Wang, Xiaoxiao Wei, Tehua Wang, et al. "Heterogeneous‐Interface‐Enhanced Adsorption of Organic and Hydroxyl for Biomass Electrooxidation." Advanced Materials 34, no. 42 (2022): e2204089. https://doi.org/10.1002/adma.202204089.
Zhou P., Lv X., Tao S. [и др.] Heterogeneous‐Interface‐Enhanced Adsorption of Organic and Hydroxyl for Biomass Electrooxidation // Advanced Materials. — 2022. — Vol. 34, № 42. — P. e2204089. — URL: https://doi.org/10.1002/adma.202204089
@article{zhou2022heterogeneousinterfaceenhanced,
title = {{Heterogeneous‐Interface‐Enhanced Adsorption of Organic and Hydroxyl for Biomass Electrooxidation}},
author = {Peng Zhou and Xingshuai Lv and Shasha Tao and Jingcheng Wu and Hongfang Wang and Xiaoxiao Wei and Tehua Wang and Bo Zhou and Yuxuan Lu and Thomas Frauenheim and Xian‐Zhu Fu and Shuangyin Wang and Yuqin Zou},
journal = {Advanced Materials},
year = {2022},
volume = {34},
number = {42},
pages = {e2204089},
doi = {10.1002/adma.202204089},
url = {https://doi.org/10.1002/adma.202204089}
}TY - JOUR AU - Zhou, Peng AU - Lv, Xingshuai AU - Tao, Shasha AU - Wu, Jingcheng AU - Wang, Hongfang AU - Wei, Xiaoxiao AU - Wang, Tehua AU - Zhou, Bo AU - Lu, Yuxuan AU - Frauenheim, Thomas AU - Fu, Xian‐Zhu AU - Wang, Shuangyin AU - Zou, Yuqin TI - Heterogeneous‐Interface‐Enhanced Adsorption of Organic and Hydroxyl for Biomass Electrooxidation JO - Advanced Materials VL - 34 IS - 42 SP - e2204089 PY - 2022 DA - 2022/08/29 DO - 10.1002/adma.202204089 UR - https://doi.org/10.1002/adma.202204089 ER -
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