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Yan Zhang, Long Jiao, Weijie Yang, Chenfan Xie, Hai‐Long Jiang
Single‐atom catalysts (SACs) have attracted tremendous interests due to their ultrahigh activity and selectivity. However, the rational control over coordination microenvironment of SACs remains a grand challenge. Herein, a post‐synthetic metal substitution (PSMS) strategy has been developed to fabricate single‐atom Ni catalysts with different N coordination numbers (denoted Ni‐Nx‐C) on pre‐designed N‐doped carbon derived from metal‐organic frameworks. When served for CO2 electroreduction, the obtained Ni‐N3‐C catalyst achieves CO Faradaic efficiency (FE) up to 95.6 %, much superior to that of Ni‐N4‐C. Theoretical calculations reveal that the lower Ni coordination number in Ni‐N3‐C can significantly enhance COOH* formation, thereby accelerating CO2 reduction. In addition, Ni‐N3‐C shows excellent performance in Zn–CO2 battery with ultrahigh CO FE and excellent stability. This work opens up a new and general avenue to coordination microenvironment modulation (MEM) of SACs for CO2 utilization.
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Zhang, Y., Jiao, L., Yang, W., Xie, C., & Jiang, H. (2021). Rational Fabrication of Low‐Coordinate Single‐Atom Ni Electrocatalysts by MOFs for Highly Selective CO2 Reduction. Angewandte Chemie International Edition, 60(14), 7607–7611. https://doi.org/10.1002/anie.202016219
Zhang, Yan, et al. "Rational Fabrication of Low‐Coordinate Single‐Atom Ni Electrocatalysts by MOFs for Highly Selective CO2 Reduction." Angewandte Chemie International Edition, vol. 60, no. 14, 2021, pp. 7607–7611, https://doi.org/10.1002/anie.202016219.
Zhang, Yan, Long Jiao, Weijie Yang, Chenfan Xie, and Hai‐Long Jiang. "Rational Fabrication of Low‐Coordinate Single‐Atom Ni Electrocatalysts by MOFs for Highly Selective CO2 Reduction." Angewandte Chemie International Edition 60, no. 14 (2021): 7607–7611. https://doi.org/10.1002/anie.202016219.
Zhang Y., Jiao L., Yang W. [и др.] Rational Fabrication of Low‐Coordinate Single‐Atom Ni Electrocatalysts by MOFs for Highly Selective CO2 Reduction // Angewandte Chemie International Edition. — 2021. — Vol. 60, № 14. — P. 7607–7611. — URL: https://doi.org/10.1002/anie.202016219
@article{zhang2021rational,
title = {{Rational Fabrication of Low‐Coordinate Single‐Atom Ni Electrocatalysts by MOFs for Highly Selective CO2 Reduction}},
author = {Yan Zhang and Long Jiao and Weijie Yang and Chenfan Xie and Hai‐Long Jiang},
journal = {Angewandte Chemie International Edition},
year = {2021},
volume = {60},
number = {14},
pages = {7607--7611},
doi = {10.1002/anie.202016219},
url = {https://doi.org/10.1002/anie.202016219}
}TY - JOUR AU - Zhang, Yan AU - Jiao, Long AU - Yang, Weijie AU - Xie, Chenfan AU - Jiang, Hai‐Long TI - Rational Fabrication of Low‐Coordinate Single‐Atom Ni Electrocatalysts by MOFs for Highly Selective CO2 Reduction JO - Angewandte Chemie International Edition VL - 60 IS - 14 SP - 7607 EP - 7611 PY - 2021 DA - 2021/01/15 DO - 10.1002/anie.202016219 UR - https://doi.org/10.1002/anie.202016219 ER -
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