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Youssef Abderrazak, Aditya Bhattacharyya, Oliver Reiser
The mainstream applications of visible‐light photoredox catalysis predominately involve outer‐sphere single‐electron transfer (SET) or energy transfer (EnT) processes of precious metal RuII or IrIII complexes or of organic dyes with low photostability. Earth‐abundant metal‐based MnLn‐type (M=metal, Ln=polydentate ligands) complexes are rapidly evolving as alternative photocatalysts as they offer not only economic and ecological advantages but also access to the complementary inner‐sphere mechanistic modes, thereby transcending their inherent limitations of ultrashort excited‐state lifetimes for use as effective photocatalysts. The generic process, termed visible‐light‐induced homolysis (VLIH), entails the formation of suitable light‐absorbing ligated metal–substrate complexes (MnLn‐Z; Z=substrate) that can undergo homolytic cleavage to generate Mn−1Ln and Z. for further transformations.
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Abderrazak, Y., Bhattacharyya, A., & Reiser, O. (2021). Visible‐Light‐Induced Homolysis of Earth‐Abundant Metal‐Substrate Complexes: A Complementary Activation Strategy in Photoredox Catalysis. Angewandte Chemie International Edition, 60(39), 21100–21115. https://doi.org/10.1002/anie.202100270
Abderrazak, Youssef, et al. "Visible‐Light‐Induced Homolysis of Earth‐Abundant Metal‐Substrate Complexes: A Complementary Activation Strategy in Photoredox Catalysis." Angewandte Chemie International Edition, vol. 60, no. 39, 2021, pp. 21100–21115, https://doi.org/10.1002/anie.202100270.
Abderrazak, Youssef, Aditya Bhattacharyya, and Oliver Reiser. "Visible‐Light‐Induced Homolysis of Earth‐Abundant Metal‐Substrate Complexes: A Complementary Activation Strategy in Photoredox Catalysis." Angewandte Chemie International Edition 60, no. 39 (2021): 21100–21115. https://doi.org/10.1002/anie.202100270.
Abderrazak Y., Bhattacharyya A., Reiser O. Visible‐Light‐Induced Homolysis of Earth‐Abundant Metal‐Substrate Complexes: A Complementary Activation Strategy in Photoredox Catalysis // Angewandte Chemie International Edition. — 2021. — Vol. 60, № 39. — P. 21100–21115. — URL: https://doi.org/10.1002/anie.202100270
@article{abderrazak2021visiblelightinduced,
title = {{Visible‐Light‐Induced Homolysis of Earth‐Abundant Metal‐Substrate Complexes: A Complementary Activation Strategy in Photoredox Catalysis}},
author = {Youssef Abderrazak and Aditya Bhattacharyya and Oliver Reiser},
journal = {Angewandte Chemie International Edition},
year = {2021},
volume = {60},
number = {39},
pages = {21100--21115},
doi = {10.1002/anie.202100270},
url = {https://doi.org/10.1002/anie.202100270}
}TY - JOUR AU - Abderrazak, Youssef AU - Bhattacharyya, Aditya AU - Reiser, Oliver TI - Visible‐Light‐Induced Homolysis of Earth‐Abundant Metal‐Substrate Complexes: A Complementary Activation Strategy in Photoredox Catalysis JO - Angewandte Chemie International Edition VL - 60 IS - 39 SP - 21100 EP - 21115 PY - 2021 DA - 2021/02/18 DO - 10.1002/anie.202100270 UR - https://doi.org/10.1002/anie.202100270 ER -
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