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Yanan Bo, Haiyun Wang, Yunxiang Lin, Tian Yang, Run Ye, Yu Li, Canyu Hu, Pengye Du, Yangguang Hu, Zhi Liu and 6 more
To avoid the energy‐consuming step of direct N≡N bond cleavage, photocatalytic N 2 fixation undergoing the associative pathways has been developed for mild‐condition operation. However, it is a fundamental yet challenging task to gain comprehensive understanding on how the associative pathways (i.e., alternating vs. distal) are influenced and altered by the fine structure of catalysts, which eventually holds the key to significantly promote the practical implementation. Herein, we introduce Fe dopants into TiO 2 nanofibers to stabilize oxygen vacancies and simultaneously tune their local electronic structure. The combination of in situ characterizations with first‐principles simulations reveals that the modulation of local electronic structure by Fe dopants turns the hydrogenation of N 2 from associative alternating pathway to associative distal pathway. This work provides fresh hints for rationally controlling the reaction pathways toward efficient photocatalytic nitrogen fixation.
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Bo, Y., Wang, H., Lin, Y., Yang, T., Ye, R., Li, Y., Hu, C., Du, P., Hu, Y., Liu, Z., Long, R., Gao, C., Ye, B., Song, L., Wu, X., & Xiong, Y. (2021). Altering Hydrogenation Pathways in Photocatalytic Nitrogen Fixation by Tuning Local Electronic Structure of Oxygen Vacancy with Dopant. Angewandte Chemie International Edition, 60(29), 16085–16092. https://doi.org/10.1002/anie.202104001
Bo, Yanan, et al. "Altering Hydrogenation Pathways in Photocatalytic Nitrogen Fixation by Tuning Local Electronic Structure of Oxygen Vacancy with Dopant." Angewandte Chemie International Edition, vol. 60, no. 29, 2021, pp. 16085–16092, https://doi.org/10.1002/anie.202104001.
Bo, Yanan, Haiyun Wang, Yunxiang Lin, Tian Yang, Run Ye, Yu Li, Canyu Hu, et al. "Altering Hydrogenation Pathways in Photocatalytic Nitrogen Fixation by Tuning Local Electronic Structure of Oxygen Vacancy with Dopant." Angewandte Chemie International Edition 60, no. 29 (2021): 16085–16092. https://doi.org/10.1002/anie.202104001.
Bo Y., Wang H., Lin Y. [и др.] Altering Hydrogenation Pathways in Photocatalytic Nitrogen Fixation by Tuning Local Electronic Structure of Oxygen Vacancy with Dopant // Angewandte Chemie International Edition. — 2021. — Vol. 60, № 29. — P. 16085–16092. — URL: https://doi.org/10.1002/anie.202104001
@article{bo2021altering,
title = {{Altering Hydrogenation Pathways in Photocatalytic Nitrogen Fixation by Tuning Local Electronic Structure of Oxygen Vacancy with Dopant}},
author = {Yanan Bo and Haiyun Wang and Yunxiang Lin and Tian Yang and Run Ye and Yu Li and Canyu Hu and Pengye Du and Yangguang Hu and Zhi Liu and Ran Long and Chao Gao and Bangjiao Ye and Li Song and Xiaojun Wu and Yujie Xiong},
journal = {Angewandte Chemie International Edition},
year = {2021},
volume = {60},
number = {29},
pages = {16085--16092},
doi = {10.1002/anie.202104001},
url = {https://doi.org/10.1002/anie.202104001}
}TY - JOUR AU - Bo, Yanan AU - Wang, Haiyun AU - Lin, Yunxiang AU - Yang, Tian AU - Ye, Run AU - Li, Yu AU - Hu, Canyu AU - Du, Pengye AU - Hu, Yangguang AU - Liu, Zhi AU - Long, Ran AU - Gao, Chao AU - Ye, Bangjiao AU - Song, Li AU - Wu, Xiaojun AU - Xiong, Yujie TI - Altering Hydrogenation Pathways in Photocatalytic Nitrogen Fixation by Tuning Local Electronic Structure of Oxygen Vacancy with Dopant JO - Angewandte Chemie International Edition VL - 60 IS - 29 SP - 16085 EP - 16092 PY - 2021 DA - 2021/05/09 DO - 10.1002/anie.202104001 UR - https://doi.org/10.1002/anie.202104001 ER -
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