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Peng Sun, Liang Ma, Wanhai Zhou, Meijia Qiu, Zilong Wang, Dongliang Chao, Wenjie Mai
Dendrite growth and by‐products in Zn metal aqueous batteries have impeded their development as promising energy storage devices. We utilize a low‐cost additive, glucose, to modulate the typical ZnSO 4 electrolyte system for improving reversible plating/stripping on Zn anode for high‐performance Zn ion batteries (ZIBs). Combing experimental characterizations and theoretical calculations, we show that the glucose in ZnSO 4 aqueous environment can simultaneously modulate solvation structure of Zn 2+ and Zn anode‐electrolyte interface. The electrolyte engineering can alternate one H 2 O molecule from the primary Zn 2+ ‐6H 2 O solvation shell and restraining side reactions due to the decomposition of active water. Concomitantly, glucose molecules are inclined to absorb on the surface of Zn anode, suppressing the random growth of Zn dendrite. As a proof of concept, a symmetric cell and Zn‐MnO 2 full cell with glucose electrolyte achieve boosted stability than that with pure ZnSO 4 electrolyte.
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Sun, P., Ma, L., Zhou, W., Qiu, M., Wang, Z., Chao, D., & Mai, W. (2021). Simultaneous Regulation on Solvation Shell and Electrode Interface for Dendrite‐Free Zn Ion Batteries Achieved by a Low‐Cost Glucose Additive. Angewandte Chemie International Edition, 60(33), 18247–18255. https://doi.org/10.1002/anie.202105756
Sun, Peng, et al. "Simultaneous Regulation on Solvation Shell and Electrode Interface for Dendrite‐Free Zn Ion Batteries Achieved by a Low‐Cost Glucose Additive." Angewandte Chemie International Edition, vol. 60, no. 33, 2021, pp. 18247–18255, https://doi.org/10.1002/anie.202105756.
Sun, Peng, Liang Ma, Wanhai Zhou, Meijia Qiu, Zilong Wang, Dongliang Chao, and Wenjie Mai. "Simultaneous Regulation on Solvation Shell and Electrode Interface for Dendrite‐Free Zn Ion Batteries Achieved by a Low‐Cost Glucose Additive." Angewandte Chemie International Edition 60, no. 33 (2021): 18247–18255. https://doi.org/10.1002/anie.202105756.
Sun P., Ma L., Zhou W. [и др.] Simultaneous Regulation on Solvation Shell and Electrode Interface for Dendrite‐Free Zn Ion Batteries Achieved by a Low‐Cost Glucose Additive // Angewandte Chemie International Edition. — 2021. — Vol. 60, № 33. — P. 18247–18255. — URL: https://doi.org/10.1002/anie.202105756
@article{sun2021simultaneous,
title = {{Simultaneous Regulation on Solvation Shell and Electrode Interface for Dendrite‐Free Zn Ion Batteries Achieved by a Low‐Cost Glucose Additive}},
author = {Peng Sun and Liang Ma and Wanhai Zhou and Meijia Qiu and Zilong Wang and Dongliang Chao and Wenjie Mai},
journal = {Angewandte Chemie International Edition},
year = {2021},
volume = {60},
number = {33},
pages = {18247--18255},
doi = {10.1002/anie.202105756},
url = {https://doi.org/10.1002/anie.202105756}
}TY - JOUR AU - Sun, Peng AU - Ma, Liang AU - Zhou, Wanhai AU - Qiu, Meijia AU - Wang, Zilong AU - Chao, Dongliang AU - Mai, Wenjie TI - Simultaneous Regulation on Solvation Shell and Electrode Interface for Dendrite‐Free Zn Ion Batteries Achieved by a Low‐Cost Glucose Additive JO - Angewandte Chemie International Edition VL - 60 IS - 33 SP - 18247 EP - 18255 PY - 2021 DA - 2021/05/25 DO - 10.1002/anie.202105756 UR - https://doi.org/10.1002/anie.202105756 ER -
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