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Lijie Zhang, Haeseong Jang, Huihui Liu, Min Gyu Kim, Dongjiang Yang, Shangguo Liu, Xien Liu, Jaephil Cho
The oxygen evolution reaction (OER) is a key reaction for many electrochemical devices. To date, many OER electrocatalysts function well in alkaline media, but exhibit poor performances in neutral and acidic media, especially the acidic stability. Herein, sodium‐decorated amorphous/crystalline RuO 2 with rich oxygen vacancies (a/c‐RuO 2 ) was developed as a pH‐universal OER electrocatalyst. The a/c‐RuO 2 shows remarkable resistance to acid corrosion and oxidation during OER, which leads to an extremely high catalytic stability, as confirmed by a negligible overpotential increase after continuously catalyzing OER for 60 h at pH=1. Besides, a/c‐RuO 2 also exhibits superior OER activities to commercial RuO 2 and most reported OER catalysts under all pH conditions. Theoretical calculations indicated that the introduction of Na dopant and oxygen vacancy in RuO 2 weakens the adsorption strength of the OER intermediates by engineering the d ‐band center, thereby lowering the energy barrier for OER.
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Zhang, L., Jang, H., Liu, H., Kim, M. G., Yang, D., Liu, S., Liu, X., & Cho, J. (2021). Sodium‐Decorated Amorphous/Crystalline RuO 2 with Rich Oxygen Vacancies: A Robust pH‐Universal Oxygen Evolution Electrocatalyst. Angewandte Chemie International Edition, 60(34), 18821–18829. https://doi.org/10.1002/anie.202106631
Zhang, Lijie, et al. "Sodium‐Decorated Amorphous/Crystalline RuO 2 with Rich Oxygen Vacancies: A Robust pH‐Universal Oxygen Evolution Electrocatalyst." Angewandte Chemie International Edition, vol. 60, no. 34, 2021, pp. 18821–18829, https://doi.org/10.1002/anie.202106631.
Zhang, Lijie, Haeseong Jang, Huihui Liu, Min Gyu Kim, Dongjiang Yang, Shangguo Liu, Xien Liu, and Jaephil Cho. "Sodium‐Decorated Amorphous/Crystalline RuO 2 with Rich Oxygen Vacancies: A Robust pH‐Universal Oxygen Evolution Electrocatalyst." Angewandte Chemie International Edition 60, no. 34 (2021): 18821–18829. https://doi.org/10.1002/anie.202106631.
Zhang L., Jang H., Liu H. [и др.] Sodium‐Decorated Amorphous/Crystalline RuO 2 with Rich Oxygen Vacancies: A Robust pH‐Universal Oxygen Evolution Electrocatalyst // Angewandte Chemie International Edition. — 2021. — Vol. 60, № 34. — P. 18821–18829. — URL: https://doi.org/10.1002/anie.202106631
@article{zhang2021sodiumdecorated,
title = {{Sodium‐Decorated Amorphous/Crystalline RuO 2 with Rich Oxygen Vacancies: A Robust pH‐Universal Oxygen Evolution Electrocatalyst}},
author = {Lijie Zhang and Haeseong Jang and Huihui Liu and Min Gyu Kim and Dongjiang Yang and Shangguo Liu and Xien Liu and Jaephil Cho},
journal = {Angewandte Chemie International Edition},
year = {2021},
volume = {60},
number = {34},
pages = {18821--18829},
doi = {10.1002/anie.202106631},
url = {https://doi.org/10.1002/anie.202106631}
}TY - JOUR AU - Zhang, Lijie AU - Jang, Haeseong AU - Liu, Huihui AU - Kim, Min Gyu AU - Yang, Dongjiang AU - Liu, Shangguo AU - Liu, Xien AU - Cho, Jaephil TI - Sodium‐Decorated Amorphous/Crystalline RuO 2 with Rich Oxygen Vacancies: A Robust pH‐Universal Oxygen Evolution Electrocatalyst JO - Angewandte Chemie International Edition VL - 60 IS - 34 SP - 18821 EP - 18829 PY - 2021 DA - 2021/06/13 DO - 10.1002/anie.202106631 UR - https://doi.org/10.1002/anie.202106631 ER -
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