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Longshuai Zhang, Xunheng Jiang, Zi‐Ai Zhong, Lei Tian, Qing Sun, Yi‐Tao Cui, Xin Lü, Jian‐Ping Zou, Shenglian Luo
Singlet oxygen ( 1 O 2 ) is an excellent active species for the selective degradation of organic pollutions. However, it is difficult to achieve high efficiency and selectivity for the generation of 1 O 2 . In this work, we develop a graphitic carbon nitride supported Fe single‐atoms catalyst (Fe 1 /CN) containing highly uniform Fe‐N 4 active sites with a high Fe loading of 11.2 wt %. The Fe 1 /CN achieves generation of 100 % 1 O 2 by activating peroxymonosulfate (PMS), which shows an ultrahigh p‐chlorophenol degradation efficiency. Density functional theory calculations results demonstrate that in contrast to Co and Ni single‐atom sites, the Fe‐N 4 sites in Fe 1 /CN adsorb the terminal O of PMS, which can facilitate the oxidization of PMS to form SO 5 .− , and thereafter efficiently generate 1 O 2 with 100 % selectivity. In addition, the Fe 1 /CN exhibits strong resistance to inorganic ions, natural organic matter, and pH value during the degradation of organic pollutants in the presence of PMS. This work develops a novel catalyst for the 100 % selective production of 1 O 2 for highly selective and efficient degradation of pollutants.
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Zhang, L., Jiang, X., Zhong, Z., Tian, L., Sun, Q., Cui, Y., Lü, X., Zou, J., & Luo, S. (2021). Carbon Nitride Supported High‐Loading Fe Single‐Atom Catalyst for Activation of Peroxymonosulfate to Generate 1 O 2 with 100 % Selectivity. Angewandte Chemie International Edition, 60(40), 21751–21755. https://doi.org/10.1002/anie.202109488
Zhang, Longshuai, et al. "Carbon Nitride Supported High‐Loading Fe Single‐Atom Catalyst for Activation of Peroxymonosulfate to Generate 1 O 2 with 100 % Selectivity." Angewandte Chemie International Edition, vol. 60, no. 40, 2021, pp. 21751–21755, https://doi.org/10.1002/anie.202109488.
Zhang, Longshuai, Xunheng Jiang, Zi‐Ai Zhong, Lei Tian, Qing Sun, Yi‐Tao Cui, Xin Lü, Jian‐Ping Zou, and Shenglian Luo. "Carbon Nitride Supported High‐Loading Fe Single‐Atom Catalyst for Activation of Peroxymonosulfate to Generate 1 O 2 with 100 % Selectivity." Angewandte Chemie International Edition 60, no. 40 (2021): 21751–21755. https://doi.org/10.1002/anie.202109488.
Zhang L., Jiang X., Zhong Z. [и др.] Carbon Nitride Supported High‐Loading Fe Single‐Atom Catalyst for Activation of Peroxymonosulfate to Generate 1 O 2 with 100 % Selectivity // Angewandte Chemie International Edition. — 2021. — Vol. 60, № 40. — P. 21751–21755. — URL: https://doi.org/10.1002/anie.202109488
@article{zhang2021carbon,
title = {{Carbon Nitride Supported High‐Loading Fe Single‐Atom Catalyst for Activation of Peroxymonosulfate to Generate 1 O 2 with 100 \% Selectivity}},
author = {Longshuai Zhang and Xunheng Jiang and Zi‐Ai Zhong and Lei Tian and Qing Sun and Yi‐Tao Cui and Xin Lü and Jian‐Ping Zou and Shenglian Luo},
journal = {Angewandte Chemie International Edition},
year = {2021},
volume = {60},
number = {40},
pages = {21751--21755},
doi = {10.1002/anie.202109488},
url = {https://doi.org/10.1002/anie.202109488}
}TY - JOUR AU - Zhang, Longshuai AU - Jiang, Xunheng AU - Zhong, Zi‐Ai AU - Tian, Lei AU - Sun, Qing AU - Cui, Yi‐Tao AU - Lü, Xin AU - Zou, Jian‐Ping AU - Luo, Shenglian TI - Carbon Nitride Supported High‐Loading Fe Single‐Atom Catalyst for Activation of Peroxymonosulfate to Generate 1 O 2 with 100 % Selectivity JO - Angewandte Chemie International Edition VL - 60 IS - 40 SP - 21751 EP - 21755 PY - 2021 DA - 2021/08/04 DO - 10.1002/anie.202109488 UR - https://doi.org/10.1002/anie.202109488 ER -
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