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Wu‐Ji Sun, Haoqing Ji, Lan‐Xin Li, Hao‐Yu Zhang, Zhen‐Kang Wang, Jinghui He, Jianmei Lu
A built‐in electric field in electrocatalyst can significantly accumulate higher concentration of NO3− ions near electrocatalyst surface region, thus facilitating mass transfer for efficient nitrate removal at ultra‐low concentration and electroreduction reaction (NO3RR). A model electrocatalyst is created by stacking CuCl (111) and rutile TiO2 (110) layers together, in which a built‐in electric field induced from the electron transfer from TiO2 to CuCl (CuCl_BEF) is successfully formed . This built‐in electric field effectively triggers interfacial accumulation of NO3− ions around the electrocatalyst. The electric field also raises the energy of key reaction intermediate *NO to lower the energy barrier of the rate determining step. A NH3 product selectivity of 98.6 %, a low NO2− production of <0.6 %, and mass‐specific ammonia production rate of 64.4 h−1 is achieved, which are all the best among studies reported at 100 mg L−1 of nitrate concentration to date.
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Sun, W., Ji, H., Li, L., Zhang, H., Wang, Z., He, J., & Lu, J. (2021). Built‐in Electric Field Triggered Interfacial Accumulation Effect for Efficient Nitrate Removal at Ultra‐Low Concentration and Electroreduction to Ammonia. Angewandte Chemie International Edition, 60(42), 22933–22939. https://doi.org/10.1002/anie.202109785
Sun, Wu‐Ji, et al. "Built‐in Electric Field Triggered Interfacial Accumulation Effect for Efficient Nitrate Removal at Ultra‐Low Concentration and Electroreduction to Ammonia." Angewandte Chemie International Edition, vol. 60, no. 42, 2021, pp. 22933–22939, https://doi.org/10.1002/anie.202109785.
Sun, Wu‐Ji, Haoqing Ji, Lan‐Xin Li, Hao‐Yu Zhang, Zhen‐Kang Wang, Jinghui He, and Jianmei Lu. "Built‐in Electric Field Triggered Interfacial Accumulation Effect for Efficient Nitrate Removal at Ultra‐Low Concentration and Electroreduction to Ammonia." Angewandte Chemie International Edition 60, no. 42 (2021): 22933–22939. https://doi.org/10.1002/anie.202109785.
Sun W., Ji H., Li L. [и др.] Built‐in Electric Field Triggered Interfacial Accumulation Effect for Efficient Nitrate Removal at Ultra‐Low Concentration and Electroreduction to Ammonia // Angewandte Chemie International Edition. — 2021. — Vol. 60, № 42. — P. 22933–22939. — URL: https://doi.org/10.1002/anie.202109785
@article{sun2021builtin,
title = {{Built‐in Electric Field Triggered Interfacial Accumulation Effect for Efficient Nitrate Removal at Ultra‐Low Concentration and Electroreduction to Ammonia}},
author = {Wu‐Ji Sun and Haoqing Ji and Lan‐Xin Li and Hao‐Yu Zhang and Zhen‐Kang Wang and Jinghui He and Jianmei Lu},
journal = {Angewandte Chemie International Edition},
year = {2021},
volume = {60},
number = {42},
pages = {22933--22939},
doi = {10.1002/anie.202109785},
url = {https://doi.org/10.1002/anie.202109785}
}TY - JOUR AU - Sun, Wu‐Ji AU - Ji, Haoqing AU - Li, Lan‐Xin AU - Zhang, Hao‐Yu AU - Wang, Zhen‐Kang AU - He, Jinghui AU - Lu, Jianmei TI - Built‐in Electric Field Triggered Interfacial Accumulation Effect for Efficient Nitrate Removal at Ultra‐Low Concentration and Electroreduction to Ammonia JO - Angewandte Chemie International Edition VL - 60 IS - 42 SP - 22933 EP - 22939 PY - 2021 DA - 2021/08/25 DO - 10.1002/anie.202109785 UR - https://doi.org/10.1002/anie.202109785 ER -
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