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Longcheng Zhang, Jie Liang, Yuanyuan Wang, Ting Mou, Yiting Lin, Luchao Yue, Tingshuai Li, Qian Liu, Yonglan Luo, Na Li and 7 more
Electrochemical reduction of NO not only offers an attractive alternative to the Haber–Bosch process for ambient NH 3 production but mitigates the human‐caused unbalance of nitrogen cycle. Herein, we report that MoS 2 nanosheet on graphite felt (MoS 2 /GF) acts as an efficient and robust 3D electrocatalyst for NO‐to‐NH 3 conversion. In acidic electrolyte, such MoS 2 /GF attains a maximal Faradaic efficiency of 76.6 % and a large NH 3 yield of up to 99.6 μmol cm −2 h −1 . Using MoS 2 nanosheet‐loaded carbon paper as the cathode, a proof‐of‐concept device of Zn‐NO battery was assembled to deliver a discharge power density of 1.04 mW cm −2 and an NH 3 yield of 411.8 μg h −1 mg cat. −1 . Calculations reveal that the positively charged Mo‐edge sites facilitate NO adsorption/activation via an acceptance–donation mechanism and disfavor the binding of protons and the coupling of N−N bond.
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Zhang, L., Liang, J., Wang, Y., Mou, T., Lin, Y., Yue, L., Li, T., Liu, Q., Luo, Y., Li, N., Tang, B., Liu, Y., Gao, S., Alshehri, A. A., Guo, X., Ma, D., & Sun, X. (2021). High‐Performance Electrochemical NO Reduction into NH 3 by MoS 2 Nanosheet. Angewandte Chemie International Edition, 60(48), 25263–25268. https://doi.org/10.1002/anie.202110879
Zhang, Longcheng, et al. "High‐Performance Electrochemical NO Reduction into NH 3 by MoS 2 Nanosheet." Angewandte Chemie International Edition, vol. 60, no. 48, 2021, pp. 25263–25268, https://doi.org/10.1002/anie.202110879.
Zhang, Longcheng, Jie Liang, Yuanyuan Wang, Ting Mou, Yiting Lin, Luchao Yue, Tingshuai Li, et al. "High‐Performance Electrochemical NO Reduction into NH 3 by MoS 2 Nanosheet." Angewandte Chemie International Edition 60, no. 48 (2021): 25263–25268. https://doi.org/10.1002/anie.202110879.
Zhang L., Liang J., Wang Y. [и др.] High‐Performance Electrochemical NO Reduction into NH 3 by MoS 2 Nanosheet // Angewandte Chemie International Edition. — 2021. — Vol. 60, № 48. — P. 25263–25268. — URL: https://doi.org/10.1002/anie.202110879
@article{zhang2021highperformance,
title = {{High‐Performance Electrochemical NO Reduction into NH 3 by MoS 2 Nanosheet}},
author = {Longcheng Zhang and Jie Liang and Yuanyuan Wang and Ting Mou and Yiting Lin and Luchao Yue and Tingshuai Li and Qian Liu and Yonglan Luo and Na Li and Bo Tang and Yang Liu and Shuyan Gao and Abdulmohsen Ali Alshehri and Xiaodong Guo and Dongwei Ma and Xuping Sun},
journal = {Angewandte Chemie International Edition},
year = {2021},
volume = {60},
number = {48},
pages = {25263--25268},
doi = {10.1002/anie.202110879},
url = {https://doi.org/10.1002/anie.202110879}
}TY - JOUR AU - Zhang, Longcheng AU - Liang, Jie AU - Wang, Yuanyuan AU - Mou, Ting AU - Lin, Yiting AU - Yue, Luchao AU - Li, Tingshuai AU - Liu, Qian AU - Luo, Yonglan AU - Li, Na AU - Tang, Bo AU - Liu, Yang AU - Gao, Shuyan AU - Alshehri, Abdulmohsen Ali AU - Guo, Xiaodong AU - Ma, Dongwei AU - Sun, Xuping TI - High‐Performance Electrochemical NO Reduction into NH 3 by MoS 2 Nanosheet JO - Angewandte Chemie International Edition VL - 60 IS - 48 SP - 25263 EP - 25268 PY - 2021 DA - 2021/09/14 DO - 10.1002/anie.202110879 UR - https://doi.org/10.1002/anie.202110879 ER -
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