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Tingting Cui, Yun‐Peng Wang, Tong Ye, Jiao Wu, Zhiqiang Chen, Jiong Li, Yongpeng Lei, Dingsheng S. Wang, Yadong Li
Herein, a novel dual single‐atom catalyst comprising adjacent Fe‐N 4 and Mn‐N 4 sites on 2D ultrathin N‐doped carbon nanosheets with porous structure (FeMn‐DSAC) was constructed as the cathode for a flexible low‐temperature Zn‐air battery (ZAB). FeMn‐DSAC exhibits remarkable bifunctional activities for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). Control experiments and density functional theory calculations reveal that the catalytic activity arises from the cooperative effect of the Fe/Mn dual‐sites aiding *OOH dissociation as well as the porous 2D nanosheet structure promoting active sits exposure and mass transfer during the reaction process. The excellent bifunctional activity of FeMn‐DSAC enables the ZAB to operate efficiently at ultra‐low temperature of −40 °C, delivering 30 mW cm −2 peak power density and retaining up to 86 % specific capacity from the room temperature counterpart.
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Cui, T., Wang, Y., Ye, T., Wu, J., Chen, Z., Li, J., Lei, Y., Wang, D. S., & Li, Y. (2022). Engineering Dual Single‐Atom Sites on 2D Ultrathin N‐doped Carbon Nanosheets Attaining Ultra‐Low‐Temperature Zinc‐Air Battery. Angewandte Chemie International Edition, 61(12), e202115219. https://doi.org/10.1002/anie.202115219
Cui, Tingting, et al. "Engineering Dual Single‐Atom Sites on 2D Ultrathin N‐doped Carbon Nanosheets Attaining Ultra‐Low‐Temperature Zinc‐Air Battery." Angewandte Chemie International Edition, vol. 61, no. 12, 2022, pp. e202115219, https://doi.org/10.1002/anie.202115219.
Cui, Tingting, Yun‐Peng Wang, Tong Ye, Jiao Wu, Zhiqiang Chen, Jiong Li, Yongpeng Lei, Dingsheng S. Wang, and Yadong Li. "Engineering Dual Single‐Atom Sites on 2D Ultrathin N‐doped Carbon Nanosheets Attaining Ultra‐Low‐Temperature Zinc‐Air Battery." Angewandte Chemie International Edition 61, no. 12 (2022): e202115219. https://doi.org/10.1002/anie.202115219.
Cui T., Wang Y., Ye T. [и др.] Engineering Dual Single‐Atom Sites on 2D Ultrathin N‐doped Carbon Nanosheets Attaining Ultra‐Low‐Temperature Zinc‐Air Battery // Angewandte Chemie International Edition. — 2022. — Vol. 61, № 12. — P. e202115219. — URL: https://doi.org/10.1002/anie.202115219
@article{cui2022engineering,
title = {{Engineering Dual Single‐Atom Sites on 2D Ultrathin N‐doped Carbon Nanosheets Attaining Ultra‐Low‐Temperature Zinc‐Air Battery}},
author = {Tingting Cui and Yun‐Peng Wang and Tong Ye and Jiao Wu and Zhiqiang Chen and Jiong Li and Yongpeng Lei and Dingsheng S. Wang and Yadong Li},
journal = {Angewandte Chemie International Edition},
year = {2022},
volume = {61},
number = {12},
pages = {e202115219},
doi = {10.1002/anie.202115219},
url = {https://doi.org/10.1002/anie.202115219}
}TY - JOUR AU - Cui, Tingting AU - Wang, Yun‐Peng AU - Ye, Tong AU - Wu, Jiao AU - Chen, Zhiqiang AU - Li, Jiong AU - Lei, Yongpeng AU - Wang, Dingsheng S. AU - Li, Yadong TI - Engineering Dual Single‐Atom Sites on 2D Ultrathin N‐doped Carbon Nanosheets Attaining Ultra‐Low‐Temperature Zinc‐Air Battery JO - Angewandte Chemie International Edition VL - 61 IS - 12 SP - e202115219 PY - 2022 DA - 2022/01/07 DO - 10.1002/anie.202115219 UR - https://doi.org/10.1002/anie.202115219 ER -
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