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Huimin Liu, Xiuyao Lang, Chao Zhu, Janis Timoshenko, Martina Rüscher, Lichen Bai, Néstor Guijarro, Haibo Yin, Yue Peng, Junhua Li and 4 more
The electrochemical nitrate reduction reaction (NITRR) provides a promising solution for restoring the imbalance in the global nitrogen cycle while enabling a sustainable and decentralized route to source ammonia. Here, we demonstrate a novel electrocatalyst for NITRR consisting of Rh clusters and single‐atoms dispersed onto Cu nanowires (NWs), which delivers a partial current density of 162 mA cm −2 for NH 3 production and a Faradaic efficiency (FE) of 93 % at −0.2 V vs. RHE. The highest ammonia yield rate reached a record value of 1.27 mmol h −1 cm −2 . Detailed investigations by electron paramagnetic resonance, in situ infrared spectroscopy, differential electrochemical mass spectrometry and density functional theory modeling suggest that the high activity originates from the synergistic catalytic cooperation between Rh and Cu sites, whereby adsorbed hydrogen on Rh site transfers to vicinal *NO intermediate species adsorbed on Cu promoting the hydrogenation and ammonia formation.
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Liu, H., Lang, X., Zhu, C., Timoshenko, J., Rüscher, M., Bai, L., Guijarro, N., Yin, H., Peng, Y., Li, J., Liu, Z., Wang, W., Cuenya, B. R., & Luo, J. (2022). Efficient Electrochemical Nitrate Reduction to Ammonia with Copper‐Supported Rhodium Cluster and Single‐Atom Catalysts. Angewandte Chemie International Edition, 61(23), e202202556. https://doi.org/10.1002/anie.202202556
Liu, Huimin, et al. "Efficient Electrochemical Nitrate Reduction to Ammonia with Copper‐Supported Rhodium Cluster and Single‐Atom Catalysts." Angewandte Chemie International Edition, vol. 61, no. 23, 2022, pp. e202202556, https://doi.org/10.1002/anie.202202556.
Liu, Huimin, Xiuyao Lang, Chao Zhu, Janis Timoshenko, Martina Rüscher, Lichen Bai, Néstor Guijarro, et al. "Efficient Electrochemical Nitrate Reduction to Ammonia with Copper‐Supported Rhodium Cluster and Single‐Atom Catalysts." Angewandte Chemie International Edition 61, no. 23 (2022): e202202556. https://doi.org/10.1002/anie.202202556.
Liu H., Lang X., Zhu C. [и др.] Efficient Electrochemical Nitrate Reduction to Ammonia with Copper‐Supported Rhodium Cluster and Single‐Atom Catalysts // Angewandte Chemie International Edition. — 2022. — Vol. 61, № 23. — P. e202202556. — URL: https://doi.org/10.1002/anie.202202556
@article{liu2022efficient,
title = {{Efficient Electrochemical Nitrate Reduction to Ammonia with Copper‐Supported Rhodium Cluster and Single‐Atom Catalysts}},
author = {Huimin Liu and Xiuyao Lang and Chao Zhu and Janis Timoshenko and Martina Rüscher and Lichen Bai and Néstor Guijarro and Haibo Yin and Yue Peng and Junhua Li and Zheng Liu and Weichao Wang and Beatriz Roldán Cuenya and Jingshan Luo},
journal = {Angewandte Chemie International Edition},
year = {2022},
volume = {61},
number = {23},
pages = {e202202556},
doi = {10.1002/anie.202202556},
url = {https://doi.org/10.1002/anie.202202556}
}TY - JOUR AU - Liu, Huimin AU - Lang, Xiuyao AU - Zhu, Chao AU - Timoshenko, Janis AU - Rüscher, Martina AU - Bai, Lichen AU - Guijarro, Néstor AU - Yin, Haibo AU - Peng, Yue AU - Li, Junhua AU - Liu, Zheng AU - Wang, Weichao AU - Cuenya, Beatriz Roldán AU - Luo, Jingshan TI - Efficient Electrochemical Nitrate Reduction to Ammonia with Copper‐Supported Rhodium Cluster and Single‐Atom Catalysts JO - Angewandte Chemie International Edition VL - 61 IS - 23 SP - e202202556 PY - 2022 DA - 2022/03/17 DO - 10.1002/anie.202202556 UR - https://doi.org/10.1002/anie.202202556 ER -
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