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Yuting Wang, Hongjiao Li, Wei Zhou, Xi Zhang, Bin Zhang, Yifu Yu
Electrochemical reduction of nitrate pollutants to ammonia has emerged as an attractive alternative for ammonia synthesis. Currently, many strategies have been developed for enhancing nitrate reduction to ammonia (NRA) efficiency, but the influence of the degree of structural disorder is still unexplored. Here, carbon‐supported RuO2 nanosheets with adjustable crystallinity are synthesized by a facile molten salt method. The as‐synthesized amorphous RuO2 displays high ammonia Faradaic efficiency (97.46 %) and selectivity (96.42 %), greatly outperforming the crystalline counterparts. The disordered structure with abundant oxygen vacancies is revealed to modulate the d‐band center and hydrogen affinity, thus lowering the energy of the potential‐determining step (NH2*→NH3*).
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Wang, Y., Li, H., Zhou, W., Zhang, X., Zhang, B., & Yu, Y. (2022). Structurally Disordered RuO2 Nanosheets with Rich Oxygen Vacancies for Enhanced Nitrate Electroreduction to Ammonia. Angewandte Chemie International Edition, 61(19), e202202604. https://doi.org/10.1002/anie.202202604
Wang, Yuting, et al. "Structurally Disordered RuO2 Nanosheets with Rich Oxygen Vacancies for Enhanced Nitrate Electroreduction to Ammonia." Angewandte Chemie International Edition, vol. 61, no. 19, 2022, pp. e202202604, https://doi.org/10.1002/anie.202202604.
Wang, Yuting, Hongjiao Li, Wei Zhou, Xi Zhang, Bin Zhang, and Yifu Yu. "Structurally Disordered RuO2 Nanosheets with Rich Oxygen Vacancies for Enhanced Nitrate Electroreduction to Ammonia." Angewandte Chemie International Edition 61, no. 19 (2022): e202202604. https://doi.org/10.1002/anie.202202604.
Wang Y., Li H., Zhou W. [и др.] Structurally Disordered RuO2 Nanosheets with Rich Oxygen Vacancies for Enhanced Nitrate Electroreduction to Ammonia // Angewandte Chemie International Edition. — 2022. — Vol. 61, № 19. — P. e202202604. — URL: https://doi.org/10.1002/anie.202202604
@article{wang2022structurally,
title = {{Structurally Disordered RuO2 Nanosheets with Rich Oxygen Vacancies for Enhanced Nitrate Electroreduction to Ammonia}},
author = {Yuting Wang and Hongjiao Li and Wei Zhou and Xi Zhang and Bin Zhang and Yifu Yu},
journal = {Angewandte Chemie International Edition},
year = {2022},
volume = {61},
number = {19},
pages = {e202202604},
doi = {10.1002/anie.202202604},
url = {https://doi.org/10.1002/anie.202202604}
}TY - JOUR AU - Wang, Yuting AU - Li, Hongjiao AU - Zhou, Wei AU - Zhang, Xi AU - Zhang, Bin AU - Yu, Yifu TI - Structurally Disordered RuO2 Nanosheets with Rich Oxygen Vacancies for Enhanced Nitrate Electroreduction to Ammonia JO - Angewandte Chemie International Edition VL - 61 IS - 19 SP - e202202604 PY - 2022 DA - 2022/03/01 DO - 10.1002/anie.202202604 UR - https://doi.org/10.1002/anie.202202604 ER -
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