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Guike Zhang, Xiaotian Li, Kai Chen, Yali Guo, Dongwei Ma, Ke Chu
We demonstrate the great feasibility of MBenes as a new class of tandem catalysts for electrocatalytic nitrate reduction to ammonia (NO 3 RR). As a proof of concept, FeB 2 is first employed as a model MBene catalyst for the NO 3 RR, showing a maximum NH 3 ‐Faradaic efficiency of 96.8 % with a corresponding NH 3 yield of 25.5 mg h −1 cm −2 at −0.6 V vs. RHE. Mechanistic studies reveal that the exceptional NO 3 RR activity of FeB 2 arises from the tandem catalysis mechanism, that is, B sites activate NO 3 − to form intermediates, while Fe sites dissociate H 2 O and increase *H supply on B sites to promote the intermediate hydrogenation and enhance the NO 3 − ‐to‐NH 3 conversion.
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Zhang, G., Li, X., Chen, K., Guo, Y., Ma, D., & Chu, K. (2023). Tandem Electrocatalytic Nitrate Reduction to Ammonia on MBenes. Angewandte Chemie International Edition, 62(13), e202300054. https://doi.org/10.1002/anie.202300054
Zhang, Guike, et al. "Tandem Electrocatalytic Nitrate Reduction to Ammonia on MBenes." Angewandte Chemie International Edition, vol. 62, no. 13, 2023, pp. e202300054, https://doi.org/10.1002/anie.202300054.
Zhang, Guike, Xiaotian Li, Kai Chen, Yali Guo, Dongwei Ma, and Ke Chu. "Tandem Electrocatalytic Nitrate Reduction to Ammonia on MBenes." Angewandte Chemie International Edition 62, no. 13 (2023): e202300054. https://doi.org/10.1002/anie.202300054.
Zhang G., Li X., Chen K. [и др.] Tandem Electrocatalytic Nitrate Reduction to Ammonia on MBenes // Angewandte Chemie International Edition. — 2023. — Vol. 62, № 13. — P. e202300054. — URL: https://doi.org/10.1002/anie.202300054
@article{zhang2023tandem,
title = {{Tandem Electrocatalytic Nitrate Reduction to Ammonia on MBenes}},
author = {Guike Zhang and Xiaotian Li and Kai Chen and Yali Guo and Dongwei Ma and Ke Chu},
journal = {Angewandte Chemie International Edition},
year = {2023},
volume = {62},
number = {13},
pages = {e202300054},
doi = {10.1002/anie.202300054},
url = {https://doi.org/10.1002/anie.202300054}
}TY - JOUR AU - Zhang, Guike AU - Li, Xiaotian AU - Chen, Kai AU - Guo, Yali AU - Ma, Dongwei AU - Chu, Ke TI - Tandem Electrocatalytic Nitrate Reduction to Ammonia on MBenes JO - Angewandte Chemie International Edition VL - 62 IS - 13 SP - e202300054 PY - 2023 DA - 2023/02/03 DO - 10.1002/anie.202300054 UR - https://doi.org/10.1002/anie.202300054 ER -
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