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Yunfan Fu, Shuo Wang, Yi Wang, Pengfei Wei, Jiaqi Shao, Tianfu Liu, Guoxiong Wang, Xinhe Bao
Electrochemical conversion of nitrate (NO 3 − ) into ammonia (NH 3 ) represents a potential way for achieving carbon‐free NH 3 production while balancing the nitrogen cycle. Herein we report a high‐performance Cu nanosheets catalyst which delivers a NH 3 partial current density of 665 mA cm −2 and NH 3 yield rate of 1.41 mmol h −1 cm −2 in a flow cell at −0.59 V vs. reversible hydrogen electrode. The catalyst showed a high stability for 700 h with NH 3 Faradaic efficiency of ≈88 % at 365 mA cm −2 . In situ spectroscopy results verify that Cu nanosheets are in situ derived from the as‐prepared CuO nanosheets under electrochemical NO 3 − reduction reaction conditions. Electrochemical measurements and density functional theory calculations indicate that the high performance is attributed to the tandem interaction of Cu(100) and Cu(111) facets. The NO 2 − generated on the Cu(100) facets is subsequently hydrogenated on the Cu(111) facets, thus the tandem catalysis promotes the crucial hydrogenation of *NO to *NOH for NH 3 production.
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Fu, Y., Wang, S., Wang, Y., Wei, P., Shao, J., Liu, T., Wang, G., & Bao, X. (2023). Enhancing Electrochemical Nitrate Reduction to Ammonia over Cu Nanosheets via Facet Tandem Catalysis. Angewandte Chemie International Edition, 62(26), e202303327. https://doi.org/10.1002/anie.202303327
Fu, Yunfan, et al. "Enhancing Electrochemical Nitrate Reduction to Ammonia over Cu Nanosheets via Facet Tandem Catalysis." Angewandte Chemie International Edition, vol. 62, no. 26, 2023, pp. e202303327, https://doi.org/10.1002/anie.202303327.
Fu, Yunfan, Shuo Wang, Yi Wang, Pengfei Wei, Jiaqi Shao, Tianfu Liu, Guoxiong Wang, and Xinhe Bao. "Enhancing Electrochemical Nitrate Reduction to Ammonia over Cu Nanosheets via Facet Tandem Catalysis." Angewandte Chemie International Edition 62, no. 26 (2023): e202303327. https://doi.org/10.1002/anie.202303327.
Fu Y., Wang S., Wang Y. [и др.] Enhancing Electrochemical Nitrate Reduction to Ammonia over Cu Nanosheets via Facet Tandem Catalysis // Angewandte Chemie International Edition. — 2023. — Vol. 62, № 26. — P. e202303327. — URL: https://doi.org/10.1002/anie.202303327
@article{fu2023enhancing,
title = {{Enhancing Electrochemical Nitrate Reduction to Ammonia over Cu Nanosheets via Facet Tandem Catalysis}},
author = {Yunfan Fu and Shuo Wang and Yi Wang and Pengfei Wei and Jiaqi Shao and Tianfu Liu and Guoxiong Wang and Xinhe Bao},
journal = {Angewandte Chemie International Edition},
year = {2023},
volume = {62},
number = {26},
pages = {e202303327},
doi = {10.1002/anie.202303327},
url = {https://doi.org/10.1002/anie.202303327}
}TY - JOUR AU - Fu, Yunfan AU - Wang, Shuo AU - Wang, Yi AU - Wei, Pengfei AU - Shao, Jiaqi AU - Liu, Tianfu AU - Wang, Guoxiong AU - Bao, Xinhe TI - Enhancing Electrochemical Nitrate Reduction to Ammonia over Cu Nanosheets via Facet Tandem Catalysis JO - Angewandte Chemie International Edition VL - 62 IS - 26 SP - e202303327 PY - 2023 DA - 2023/04/29 DO - 10.1002/anie.202303327 UR - https://doi.org/10.1002/anie.202303327 ER -
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