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Libo Wang, Bei Cheng, Liuyang Zhang, Jiaguo Yu
Reasonable design of efficient hierarchical photocatalysts has gained significant attention. Herein, a step‐scheme (S‐scheme) core‐shell TiO 2 @ZnIn 2 S 4 heterojunction is designed for photocatalytic CO 2 reduction. The optimized sample exhibits much higher CO 2 photoreduction conversion rates (the sum yield of CO, CH 3 OH, and CH 4 ) than the blank control, i.e., ZnIn 2 S 4 and TiO 2 . The improved photocatalytic performance can be attributed to the inhibited recombination of photogenerated charge carriers induced by S‐scheme heterojunction. The improvement is also attributed to the large specific surface areas and abundant active sites. Meanwhile, S‐scheme photogenerated charge transfer mechanism is testified by in situ irradiated X‐ray photoelectron spectroscopy, work function calculation, and electron paramagnetic resonance measurements. This work provides an effective strategy for designing highly efficient heterojunction photocatalysts for conversion of solar fuels.
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Wang, L., Cheng, B., Zhang, L., & Yu, J. (2021). In situ Irradiated XPS Investigation on S‐Scheme TiO 2 @ZnIn 2 S 4 Photocatalyst for Efficient Photocatalytic CO 2 Reduction. Small, 17(41), e2103447. https://doi.org/10.1002/smll.202103447
Wang, Libo, et al. "In situ Irradiated XPS Investigation on S‐Scheme TiO 2 @ZnIn 2 S 4 Photocatalyst for Efficient Photocatalytic CO 2 Reduction." Small, vol. 17, no. 41, 2021, pp. e2103447, https://doi.org/10.1002/smll.202103447.
Wang, Libo, Bei Cheng, Liuyang Zhang, and Jiaguo Yu. "In situ Irradiated XPS Investigation on S‐Scheme TiO 2 @ZnIn 2 S 4 Photocatalyst for Efficient Photocatalytic CO 2 Reduction." Small 17, no. 41 (2021): e2103447. https://doi.org/10.1002/smll.202103447.
Wang L., Cheng B., Zhang L. [и др.] In situ Irradiated XPS Investigation on S‐Scheme TiO 2 @ZnIn 2 S 4 Photocatalyst for Efficient Photocatalytic CO 2 Reduction // Small. — 2021. — Vol. 17, № 41. — P. e2103447. — URL: https://doi.org/10.1002/smll.202103447
@article{wang2021situ,
title = {{In situ Irradiated XPS Investigation on S‐Scheme TiO 2 @ZnIn 2 S 4 Photocatalyst for Efficient Photocatalytic CO 2 Reduction}},
author = {Libo Wang and Bei Cheng and Liuyang Zhang and Jiaguo Yu},
journal = {Small},
year = {2021},
volume = {17},
number = {41},
pages = {e2103447},
doi = {10.1002/smll.202103447},
url = {https://doi.org/10.1002/smll.202103447}
}TY - JOUR AU - Wang, Libo AU - Cheng, Bei AU - Zhang, Liuyang AU - Yu, Jiaguo TI - In situ Irradiated XPS Investigation on S‐Scheme TiO 2 @ZnIn 2 S 4 Photocatalyst for Efficient Photocatalytic CO 2 Reduction JO - Small VL - 17 IS - 41 SP - e2103447 PY - 2021 DA - 2021/09/12 DO - 10.1002/smll.202103447 UR - https://doi.org/10.1002/smll.202103447 ER -
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