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Òscar Pàmies, Jèssica Margalef, Santiago Cañellas, Jinju James, Eric Judge, Patrick J. Guiry, Christina Moberg, Jan‐E. Bäckvall, Andreas Pfaltz, Miquel À. Pericàs, Montserrat Diéguez
This Review compiles the evolution, mechanistic understanding, and more recent advances in enantioselective Pd-catalyzed allylic substitution and decarboxylative and oxidative allylic substitutions. For each reaction, the catalytic data, as well as examples of their application to the synthesis of more complex molecules, are collected. Sections in which we discuss key mechanistic aspects for high selectivity and a comparison with other metals (with advantages and disadvantages) are also included. For Pd-catalyzed asymmetric allylic substitution, the catalytic data are grouped according to the type of nucleophile employed. Because of the prominent position of the use of stabilized carbon nucleophiles and heteronucleophiles, many chiral ligands have been developed. To better compare the results, they are presented grouped by ligand types. Pd-catalyzed asymmetric decarboxylative reactions are mainly promoted by PHOX or Trost ligands, which justifies organizing this section in chronological order. For asymmetric oxidative allylic substitution the results are grouped according to the type of nucleophile used.
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Pàmies, Ò., Margalef, J., Cañellas, S., James, J., Judge, E., Guiry, P. J., Moberg, C., Bäckvall, J., Pfaltz, A., Pericàs, M. À., & Diéguez, M. (2021). Recent Advances in Enantioselective Pd-Catalyzed Allylic Substitution: From Design to Applications. Chemical Reviews, 121(8), 4373–4505. https://doi.org/10.1021/acs.chemrev.0c00736
Pàmies, Òscar, et al. "Recent Advances in Enantioselective Pd-Catalyzed Allylic Substitution: From Design to Applications." Chemical Reviews, vol. 121, no. 8, 2021, pp. 4373–4505, https://doi.org/10.1021/acs.chemrev.0c00736.
Pàmies, Òscar, Jèssica Margalef, Santiago Cañellas, Jinju James, Eric Judge, Patrick J. Guiry, Christina Moberg, et al. "Recent Advances in Enantioselective Pd-Catalyzed Allylic Substitution: From Design to Applications." Chemical Reviews 121, no. 8 (2021): 4373–4505. https://doi.org/10.1021/acs.chemrev.0c00736.
Pàmies Ò., Margalef J., Cañellas S. [и др.] Recent Advances in Enantioselective Pd-Catalyzed Allylic Substitution: From Design to Applications // Chemical Reviews. — 2021. — Vol. 121, № 8. — P. 4373–4505. — URL: https://doi.org/10.1021/acs.chemrev.0c00736
@article{pamies2021recent,
title = {{Recent Advances in Enantioselective Pd-Catalyzed Allylic Substitution: From Design to Applications}},
author = {Òscar Pàmies and Jèssica Margalef and Santiago Cañellas and Jinju James and Eric Judge and Patrick J. Guiry and Christina Moberg and Jan‐E. Bäckvall and Andreas Pfaltz and Miquel À. Pericàs and Montserrat Diéguez},
journal = {Chemical Reviews},
year = {2021},
volume = {121},
number = {8},
pages = {4373--4505},
doi = {10.1021/acs.chemrev.0c00736},
url = {https://doi.org/10.1021/acs.chemrev.0c00736}
}TY - JOUR AU - Pàmies, Òscar AU - Margalef, Jèssica AU - Cañellas, Santiago AU - James, Jinju AU - Judge, Eric AU - Guiry, Patrick J. AU - Moberg, Christina AU - Bäckvall, Jan‐E. AU - Pfaltz, Andreas AU - Pericàs, Miquel À. AU - Diéguez, Montserrat TI - Recent Advances in Enantioselective Pd-Catalyzed Allylic Substitution: From Design to Applications JO - Chemical Reviews VL - 121 IS - 8 SP - 4373 EP - 4505 PY - 2021 DA - 2021/03/19 DO - 10.1021/acs.chemrev.0c00736 UR - https://doi.org/10.1021/acs.chemrev.0c00736 ER -
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