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Ning Zheng, Yang Xu, Qian Zhao, Tao Xie
Dynamic covalent polymer networks (DCPN) have historically attracted attention for their unique roles in chemical recycling and self-healing, which are both relevant for sustainable societal development. Efforts in these directions have intensified in the past decade with notable progress in newly discovered dynamic covalent chemistry, fundamental material concepts, and extension toward emerging applications including energy and electronic devices. Beyond that, the values of DCPN in discovering/designing functional properties not offered by classical thermoplastic and thermoset polymers have recently gained traction. In particular, the dynamic bond exchangeability of DCPN has shown unparalleled design versatility in various areas including shape-shifting materials/devices, artificial muscles, and microfabrication. Going beyond this basic bond exchangeability, various molecular mechanisms to manipulate network topologies (topological transformation) have led to opportunities to program polymers, with notable concepts such as living networks and topological isomerization. In this review, we provide an overview of the above progress with particular focuses on molecular design strategies for the exploitation of functional material properties. Based on this, we point out the remaining issues and offer perspectives on how this class of materials can shape the future in ways that are complementary with classical thermoplastic and thermoset polymers.
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Zheng, N., Xu, Y., Zhao, Q., & Xie, T. (2021). Dynamic Covalent Polymer Networks: A Molecular Platform for Designing Functions beyond Chemical Recycling and Self-Healing. Chemical Reviews, 121(3), 1716–1745. https://doi.org/10.1021/acs.chemrev.0c00938
Zheng, Ning, et al. "Dynamic Covalent Polymer Networks: A Molecular Platform for Designing Functions beyond Chemical Recycling and Self-Healing." Chemical Reviews, vol. 121, no. 3, 2021, pp. 1716–1745, https://doi.org/10.1021/acs.chemrev.0c00938.
Zheng, Ning, Yang Xu, Qian Zhao, and Tao Xie. "Dynamic Covalent Polymer Networks: A Molecular Platform for Designing Functions beyond Chemical Recycling and Self-Healing." Chemical Reviews 121, no. 3 (2021): 1716–1745. https://doi.org/10.1021/acs.chemrev.0c00938.
Zheng N., Xu Y., Zhao Q. [и др.] Dynamic Covalent Polymer Networks: A Molecular Platform for Designing Functions beyond Chemical Recycling and Self-Healing // Chemical Reviews. — 2021. — Vol. 121, № 3. — P. 1716–1745. — URL: https://doi.org/10.1021/acs.chemrev.0c00938
@article{zheng2021dynamic,
title = {{Dynamic Covalent Polymer Networks: A Molecular Platform for Designing Functions beyond Chemical Recycling and Self-Healing}},
author = {Ning Zheng and Yang Xu and Qian Zhao and Tao Xie},
journal = {Chemical Reviews},
year = {2021},
volume = {121},
number = {3},
pages = {1716--1745},
doi = {10.1021/acs.chemrev.0c00938},
url = {https://doi.org/10.1021/acs.chemrev.0c00938}
}TY - JOUR AU - Zheng, Ning AU - Xu, Yang AU - Zhao, Qian AU - Xie, Tao TI - Dynamic Covalent Polymer Networks: A Molecular Platform for Designing Functions beyond Chemical Recycling and Self-Healing JO - Chemical Reviews VL - 121 IS - 3 SP - 1716 EP - 1745 PY - 2021 DA - 2021/01/04 DO - 10.1021/acs.chemrev.0c00938 UR - https://doi.org/10.1021/acs.chemrev.0c00938 ER -
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