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Hui Ding, Hongfei Liu, Wangsheng Chu, Changzheng Wu, Yi Xie
Electrochemical water splitting for hydrogen generation is a promising pathway for renewable energy conversion and storage. One of the most important issues for efficient water splitting is to develop cost-effective and highly efficient electrocatalysts to drive sluggish oxygen-evolution reaction (OER) at the anode side. Notably, structural transformation such as surface oxidation of metals or metal nonoxide compounds and surface amorphization of some metal oxides during OER have attracted growing attention in recent years. The investigation of structural transformation in OER will contribute to the in-depth understanding of accurate catalytic mechanisms and will finally benefit the rational design of catalytic materials with high activity. In this Review, we provide an overview of heterogeneous materials with obvious structural transformation during OER electrocatalysis. To gain insight into the essence of structural transformation, we summarize the driving forces and critical factors that affect the transformation process. In addition, advanced techniques that are used to probe chemical states and atomic structures of transformed surfaces are also introduced. We then discuss the structure of active species and the relationship between catalytic performance and structural properties of transformed materials. Finally, the challenges and prospects of heterogeneous OER electrocatalysis are presented.
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Ding, H., Liu, H., Chu, W., Wu, C., & Xie, Y. (2021). Structural Transformation of Heterogeneous Materials for Electrocatalytic Oxygen Evolution Reaction. Chemical Reviews, 121(21), 13174–13212. https://doi.org/10.1021/acs.chemrev.1c00234
Ding, Hui, et al. "Structural Transformation of Heterogeneous Materials for Electrocatalytic Oxygen Evolution Reaction." Chemical Reviews, vol. 121, no. 21, 2021, pp. 13174–13212, https://doi.org/10.1021/acs.chemrev.1c00234.
Ding, Hui, Hongfei Liu, Wangsheng Chu, Changzheng Wu, and Yi Xie. "Structural Transformation of Heterogeneous Materials for Electrocatalytic Oxygen Evolution Reaction." Chemical Reviews 121, no. 21 (2021): 13174–13212. https://doi.org/10.1021/acs.chemrev.1c00234.
Ding H., Liu H., Chu W. [и др.] Structural Transformation of Heterogeneous Materials for Electrocatalytic Oxygen Evolution Reaction // Chemical Reviews. — 2021. — Vol. 121, № 21. — P. 13174–13212. — URL: https://doi.org/10.1021/acs.chemrev.1c00234
@article{ding2021structural,
title = {{Structural Transformation of Heterogeneous Materials for Electrocatalytic Oxygen Evolution Reaction}},
author = {Hui Ding and Hongfei Liu and Wangsheng Chu and Changzheng Wu and Yi Xie},
journal = {Chemical Reviews},
year = {2021},
volume = {121},
number = {21},
pages = {13174--13212},
doi = {10.1021/acs.chemrev.1c00234},
url = {https://doi.org/10.1021/acs.chemrev.1c00234}
}TY - JOUR AU - Ding, Hui AU - Liu, Hongfei AU - Chu, Wangsheng AU - Wu, Changzheng AU - Xie, Yi TI - Structural Transformation of Heterogeneous Materials for Electrocatalytic Oxygen Evolution Reaction JO - Chemical Reviews VL - 121 IS - 21 SP - 13174 EP - 13212 PY - 2021 DA - 2021/09/15 DO - 10.1021/acs.chemrev.1c00234 UR - https://doi.org/10.1021/acs.chemrev.1c00234 ER -
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