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Guorui Cai, Peng Yan, Liangliang Zhang, Hong-Cai “Joe” Zhou, Hai‐Long Jiang
Metal-organic frameworks (MOFs) have been widely recognized as one of the most fascinating classes of materials from science and engineering perspectives, benefiting from their high porosity and well-defined and tailored structures and components at the atomic level. Although their intrinsic micropores endow size-selective capability and high surface area, etc., the narrow pores limit their applications toward diffusion-control and large-size species involved processes. In recent years, the construction of hierarchically porous MOFs (HP-MOFs), MOF-based hierarchically porous composites, and MOF-based hierarchically porous derivatives has captured widespread interest to extend the applications of conventional MOF-based materials. In this Review, the recent advances in the design, synthesis, and functional applications of MOF-based hierarchically porous materials are summarized. Their structural characters toward various applications, including catalysis, gas storage and separation, air filtration, sewage treatment, sensing and energy storage, have been demonstrated with typical reports. The comparison of HP-MOFs with traditional porous materials (e.g., zeolite, porous silica, carbons, metal oxides, and polymers), subsisting challenges, as well as future directions in this research field, are also indicated.
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Cai, G., Yan, P., Zhang, L., Zhou, H.-C. “., & Jiang, H. (2021). Metal–Organic Framework-Based Hierarchically Porous Materials: Synthesis and Applications. Chemical Reviews, 121(20), 12278–12326. https://doi.org/10.1021/acs.chemrev.1c00243
Cai, Guorui, et al. "Metal–Organic Framework-Based Hierarchically Porous Materials: Synthesis and Applications." Chemical Reviews, vol. 121, no. 20, 2021, pp. 12278–12326, https://doi.org/10.1021/acs.chemrev.1c00243.
Cai, Guorui, Peng Yan, Liangliang Zhang, Hong-Cai “Joe” Zhou, and Hai‐Long Jiang. "Metal–Organic Framework-Based Hierarchically Porous Materials: Synthesis and Applications." Chemical Reviews 121, no. 20 (2021): 12278–12326. https://doi.org/10.1021/acs.chemrev.1c00243.
Cai G., Yan P., Zhang L. [и др.] Metal–Organic Framework-Based Hierarchically Porous Materials: Synthesis and Applications // Chemical Reviews. — 2021. — Vol. 121, № 20. — P. 12278–12326. — URL: https://doi.org/10.1021/acs.chemrev.1c00243
@article{cai2021metalorganic,
title = {{Metal–Organic Framework-Based Hierarchically Porous Materials: Synthesis and Applications}},
author = {Guorui Cai and Peng Yan and Liangliang Zhang and Hong-Cai “Joe” Zhou and Hai‐Long Jiang},
journal = {Chemical Reviews},
year = {2021},
volume = {121},
number = {20},
pages = {12278--12326},
doi = {10.1021/acs.chemrev.1c00243},
url = {https://doi.org/10.1021/acs.chemrev.1c00243}
}TY - JOUR AU - Cai, Guorui AU - Yan, Peng AU - Zhang, Liangliang AU - Zhou, Hong-Cai “Joe” AU - Jiang, Hai‐Long TI - Metal–Organic Framework-Based Hierarchically Porous Materials: Synthesis and Applications JO - Chemical Reviews VL - 121 IS - 20 SP - 12278 EP - 12326 PY - 2021 DA - 2021/07/19 DO - 10.1021/acs.chemrev.1c00243 UR - https://doi.org/10.1021/acs.chemrev.1c00243 ER -
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