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Liang Chang, Qing An, Lingfei Duan, Kaixuan Feng, Zhiwei Zuo
Alkoxy radicals are highly reactive species that have long been recognized as versatile intermediates in organic synthesis. However, their development has long been impeded due to a lack of convenient methods for their generation. Thanks to advances in photoredox catalysis, enabling facile access to alkoxy radicals from bench-stable precursors and free alcohols under mild conditions, research interest in this field has been renewed. This review comprehensively summarizes the recent progress in alkoxy radical-mediated transformations under visible light irradiation. Elementary steps for alkoxy radical generation from either radical precursors or free alcohols are central to reaction development; thus, each section is categorized and discussed accordingly. Throughout this review, we have focused on the different mechanisms of alkoxy radical generation as well as their impact on synthetic utilizations. Notably, the catalytic generation of alkoxy radicals from abundant alcohols is still in the early stage, providing intriguing opportunities to exploit alkoxy radicals for diverse synthetic paradigms.
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Chang, L., An, Q., Duan, L., Feng, K., & Zuo, Z. (2021). Alkoxy Radicals See the Light: New Paradigms of Photochemical Synthesis. Chemical Reviews, 122(2), 2429–2486. https://doi.org/10.1021/acs.chemrev.1c00256
Chang, Liang, et al. "Alkoxy Radicals See the Light: New Paradigms of Photochemical Synthesis." Chemical Reviews, vol. 122, no. 2, 2021, pp. 2429–2486, https://doi.org/10.1021/acs.chemrev.1c00256.
Chang, Liang, Qing An, Lingfei Duan, Kaixuan Feng, and Zhiwei Zuo. "Alkoxy Radicals See the Light: New Paradigms of Photochemical Synthesis." Chemical Reviews 122, no. 2 (2021): 2429–2486. https://doi.org/10.1021/acs.chemrev.1c00256.
Chang L., An Q., Duan L. [и др.] Alkoxy Radicals See the Light: New Paradigms of Photochemical Synthesis // Chemical Reviews. — 2021. — Vol. 122, № 2. — P. 2429–2486. — URL: https://doi.org/10.1021/acs.chemrev.1c00256
@article{chang2021alkoxy,
title = {{Alkoxy Radicals See the Light: New Paradigms of Photochemical Synthesis}},
author = {Liang Chang and Qing An and Lingfei Duan and Kaixuan Feng and Zhiwei Zuo},
journal = {Chemical Reviews},
year = {2021},
volume = {122},
number = {2},
pages = {2429--2486},
doi = {10.1021/acs.chemrev.1c00256},
url = {https://doi.org/10.1021/acs.chemrev.1c00256}
}TY - JOUR AU - Chang, Liang AU - An, Qing AU - Duan, Lingfei AU - Feng, Kaixuan AU - Zuo, Zhiwei TI - Alkoxy Radicals See the Light: New Paradigms of Photochemical Synthesis JO - Chemical Reviews VL - 122 IS - 2 SP - 2429 EP - 2486 PY - 2021 DA - 2021/10/06 DO - 10.1021/acs.chemrev.1c00256 UR - https://doi.org/10.1021/acs.chemrev.1c00256 ER -
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