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Bin Liu, Andrew M. Romine, Camille Rubel, Keary M. Engle, Bing‐Feng Shi
Transition-metal-catalyzed, coordination-assisted C(sp 3 )–H functionalization has revolutionized synthetic planning over the past few decades as the use of these directing groups has allowed for increased access to many strategic positions in organic molecules. Nonetheless, several challenges remain preeminent, such as the requirement for high temperatures, the difficulty in removing or converting directing groups, and, although many metals provide some reactivity, the difficulty in employing metals outside of palladium. This review aims to give a comprehensive overview of coordination-assisted, transition-metal-catalyzed, direct functionalization of nonactivated C(sp 3 )–H bonds by covering the literature since 2004 in order to demonstrate the current state-of-the-art methods as well as the current limitations. For clarity, this review has been divided into nine sections by the transition metal catalyst with subdivisions by the type of bond formation. Synthetic applications and reaction mechanism are discussed where appropriate.
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Liu, B., Romine, A. M., Rubel, C., Engle, K. M., & Shi, B. (2021). Transition-Metal-Catalyzed, Coordination-Assisted Functionalization of Nonactivated C(sp 3 )–H Bonds. Chemical Reviews, 121(24), 14957–15074. https://doi.org/10.1021/acs.chemrev.1c00519
Liu, Bin, et al. "Transition-Metal-Catalyzed, Coordination-Assisted Functionalization of Nonactivated C(sp 3 )–H Bonds." Chemical Reviews, vol. 121, no. 24, 2021, pp. 14957–15074, https://doi.org/10.1021/acs.chemrev.1c00519.
Liu, Bin, Andrew M. Romine, Camille Rubel, Keary M. Engle, and Bing‐Feng Shi. "Transition-Metal-Catalyzed, Coordination-Assisted Functionalization of Nonactivated C(sp 3 )–H Bonds." Chemical Reviews 121, no. 24 (2021): 14957–15074. https://doi.org/10.1021/acs.chemrev.1c00519.
Liu B., Romine A. M., Rubel C. [и др.] Transition-Metal-Catalyzed, Coordination-Assisted Functionalization of Nonactivated C(sp 3 )–H Bonds // Chemical Reviews. — 2021. — Vol. 121, № 24. — P. 14957–15074. — URL: https://doi.org/10.1021/acs.chemrev.1c00519
@article{liu2021transitionmetalcatalyzed,
title = {{Transition-Metal-Catalyzed, Coordination-Assisted Functionalization of Nonactivated C(sp 3 )–H Bonds}},
author = {Bin Liu and Andrew M. Romine and Camille Rubel and Keary M. Engle and Bing‐Feng Shi},
journal = {Chemical Reviews},
year = {2021},
volume = {121},
number = {24},
pages = {14957--15074},
doi = {10.1021/acs.chemrev.1c00519},
url = {https://doi.org/10.1021/acs.chemrev.1c00519}
}TY - JOUR AU - Liu, Bin AU - Romine, Andrew M. AU - Rubel, Camille AU - Engle, Keary M. AU - Shi, Bing‐Feng TI - Transition-Metal-Catalyzed, Coordination-Assisted Functionalization of Nonactivated C(sp 3 )–H Bonds JO - Chemical Reviews VL - 121 IS - 24 SP - 14957 EP - 15074 PY - 2021 DA - 2021/10/29 DO - 10.1021/acs.chemrev.1c00519 UR - https://doi.org/10.1021/acs.chemrev.1c00519 ER -
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