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Nicholas F. Dummer, David J. Willock, Qian He, Mark J. Howard, Richard J. Lewis, Guodong Qi, Stuart H. Taylor, Jun Xu, Donald Bethell, Christopher J. Kiely, Graham John Hutchings
The direct transformation of methane to methanol remains a significant challenge for operation at a larger scale. Central to this challenge is the low reactivity of methane at conditions that can facilitate product recovery. This review discusses the issue through examination of several promising routes to methanol and an evaluation of performance targets that are required to develop the process at scale. We explore the methods currently used, the emergence of active heterogeneous catalysts and their design and reaction mechanisms and provide a critical perspective on future operation. Initial experiments are discussed where identification of gas phase radical chemistry limited further development by this approach. Subsequently, a new class of catalytic materials based on natural systems such as iron or copper containing zeolites were explored at milder conditions. The key issues of these technologies are low methane conversion and often significant overoxidation of products. Despite this, interest remains high in this reaction and the wider appeal of an effective route to key products from C-H activation, particularly with the need to transition to net carbon zero with new routes from renewable methane sources is exciting.
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Dummer, N. F., Willock, D. J., He, Q., Howard, M. J., Lewis, R. J., Qi, G., Taylor, S. H., Xu, J., Bethell, D., Kiely, C. J., & Hutchings, G. J. (2022). Methane Oxidation to Methanol. Chemical Reviews, 123(9), 6359–6411. https://doi.org/10.1021/acs.chemrev.2c00439
Dummer, Nicholas F., et al. "Methane Oxidation to Methanol." Chemical Reviews, vol. 123, no. 9, 2022, pp. 6359–6411, https://doi.org/10.1021/acs.chemrev.2c00439.
Dummer, Nicholas F., David J. Willock, Qian He, Mark J. Howard, Richard J. Lewis, Guodong Qi, Stuart H. Taylor, et al. "Methane Oxidation to Methanol." Chemical Reviews 123, no. 9 (2022): 6359–6411. https://doi.org/10.1021/acs.chemrev.2c00439.
Dummer N. F., Willock D. J., He Q. [и др.] Methane Oxidation to Methanol // Chemical Reviews. — 2022. — Vol. 123, № 9. — P. 6359–6411. — URL: https://doi.org/10.1021/acs.chemrev.2c00439
@article{dummer2022methane,
title = {{Methane Oxidation to Methanol}},
author = {Nicholas F. Dummer and David J. Willock and Qian He and Mark J. Howard and Richard J. Lewis and Guodong Qi and Stuart H. Taylor and Jun Xu and Donald Bethell and Christopher J. Kiely and Graham John Hutchings},
journal = {Chemical Reviews},
year = {2022},
volume = {123},
number = {9},
pages = {6359--6411},
doi = {10.1021/acs.chemrev.2c00439},
url = {https://doi.org/10.1021/acs.chemrev.2c00439}
}TY - JOUR AU - Dummer, Nicholas F. AU - Willock, David J. AU - He, Qian AU - Howard, Mark J. AU - Lewis, Richard J. AU - Qi, Guodong AU - Taylor, Stuart H. AU - Xu, Jun AU - Bethell, Donald AU - Kiely, Christopher J. AU - Hutchings, Graham John TI - Methane Oxidation to Methanol JO - Chemical Reviews VL - 123 IS - 9 SP - 6359 EP - 6411 PY - 2022 DA - 2022/12/02 DO - 10.1021/acs.chemrev.2c00439 UR - https://doi.org/10.1021/acs.chemrev.2c00439 ER -
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