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Peter Bellotti, Huan‐Ming Huang, Teresa Faber, Frank Glorius
The emergence of modern photocatalysis, characterized by mildness and selectivity, has significantly spurred innovative late-stage C-H functionalization approaches that make use of low energy photons as a controllable energy source. Compared to traditional late-stage functionalization strategies, photocatalysis paves the way toward complementary and/or previously unattainable regio- and chemoselectivities. Merging the compelling benefits of photocatalysis with the late-stage functionalization workflow offers a potentially unmatched arsenal to tackle drug development campaigns and beyond. This Review highlights the photocatalytic late-stage C-H functionalization strategies of small-molecule drugs, agrochemicals, and natural products, classified according to the targeted C-H bond and the newly formed one. Emphasis is devoted to identifying, describing, and comparing the main mechanistic scenarios. The Review draws a critical comparison between established ionic chemistry and photocatalyzed radical-based manifolds. The Review aims to establish the current state-of-the-art and illustrate the key unsolved challenges to be addressed in the future. The authors aim to introduce the general readership to the main approaches toward photocatalytic late-stage C-H functionalization, and specialist practitioners to the critical evaluation of the current methodologies, potential for improvement, and future uncharted directions.
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Bellotti, P., Huang, H., Faber, T., & Glorius, F. (2023). Photocatalytic Late-Stage C–H Functionalization. Chemical Reviews, 123(8), 4237–4352. https://doi.org/10.1021/acs.chemrev.2c00478
Bellotti, Peter, et al. "Photocatalytic Late-Stage C–H Functionalization." Chemical Reviews, vol. 123, no. 8, 2023, pp. 4237–4352, https://doi.org/10.1021/acs.chemrev.2c00478.
Bellotti, Peter, Huan‐Ming Huang, Teresa Faber, and Frank Glorius. "Photocatalytic Late-Stage C–H Functionalization." Chemical Reviews 123, no. 8 (2023): 4237–4352. https://doi.org/10.1021/acs.chemrev.2c00478.
Bellotti P., Huang H., Faber T. [и др.] Photocatalytic Late-Stage C–H Functionalization // Chemical Reviews. — 2023. — Vol. 123, № 8. — P. 4237–4352. — URL: https://doi.org/10.1021/acs.chemrev.2c00478
@article{bellotti2023photocatalytic,
title = {{Photocatalytic Late-Stage C–H Functionalization}},
author = {Peter Bellotti and Huan‐Ming Huang and Teresa Faber and Frank Glorius},
journal = {Chemical Reviews},
year = {2023},
volume = {123},
number = {8},
pages = {4237--4352},
doi = {10.1021/acs.chemrev.2c00478},
url = {https://doi.org/10.1021/acs.chemrev.2c00478}
}TY - JOUR AU - Bellotti, Peter AU - Huang, Huan‐Ming AU - Faber, Teresa AU - Glorius, Frank TI - Photocatalytic Late-Stage C–H Functionalization JO - Chemical Reviews VL - 123 IS - 8 SP - 4237 EP - 4352 PY - 2023 DA - 2023/01/24 DO - 10.1021/acs.chemrev.2c00478 UR - https://doi.org/10.1021/acs.chemrev.2c00478 ER -
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