One connector, four scholarly indexes, real DOIs and legal free PDFs. Works in Claude and ChatGPT.
Paste it into Claude or ChatGPT as a custom connector. 3-day free trial.
Konstantijn T. Rommens, Mark Saeys
For nearly a century, the Fischer–Tropsch (FT) reaction has been subject of intense debate. Various molecular views on the active sites and on the reaction mechanism have been presented for both Co- and Fe-based FT reactions. In the last 15 years, the emergence of a surface-science- and molecular-modeling-based bottom-up approach has brought this molecular picture a step closer. Theoretical models provided a structural picture of the Co catalyst particles. Recent surface science experiments and density functional theory (DFT) calculations highlighted the importance of realistic surface coverages, which can induce surface reconstruction and impact the stability of reaction intermediates. For Co-based FTS, detailed microkinetic simulations and mechanistic experiments are moving toward a consensus about the active sites and the reaction mechanism. The dynamic phase evolution of Fe-based catalysts under the reaction conditions complicates identification of the surface structure and the active sites. New techniques can help tackle the combinatorial complexity in these systems. Experimental and DFT studies have addressed the mechanism for Fe-based catalysts; the absence of a clear molecular picture of the active sites, however, limits the development of a molecular view of the mechanism. Finally, direct CO 2 hydrogenation to long-chain hydrocarbons could present a sustainable pathway for FT synthesis.
Formatted from the source metadata, not typed by hand. For a whole reference list, use the citation generator or ask your assistant through Find Research.
Rommens, K. T., & Saeys, M. (2023). Molecular Views on Fischer–Tropsch Synthesis. Chemical Reviews, 123(9), 5798–5858. https://doi.org/10.1021/acs.chemrev.2c00508
Rommens, Konstantijn T., and Mark Saeys. "Molecular Views on Fischer–Tropsch Synthesis." Chemical Reviews, vol. 123, no. 9, 2023, pp. 5798–5858, https://doi.org/10.1021/acs.chemrev.2c00508.
Rommens, Konstantijn T., and Mark Saeys. "Molecular Views on Fischer–Tropsch Synthesis." Chemical Reviews 123, no. 9 (2023): 5798–5858. https://doi.org/10.1021/acs.chemrev.2c00508.
Rommens K. T., Saeys M. Molecular Views on Fischer–Tropsch Synthesis // Chemical Reviews. — 2023. — Vol. 123, № 9. — P. 5798–5858. — URL: https://doi.org/10.1021/acs.chemrev.2c00508
@article{rommens2023molecular,
title = {{Molecular Views on Fischer–Tropsch Synthesis}},
author = {Konstantijn T. Rommens and Mark Saeys},
journal = {Chemical Reviews},
year = {2023},
volume = {123},
number = {9},
pages = {5798--5858},
doi = {10.1021/acs.chemrev.2c00508},
url = {https://doi.org/10.1021/acs.chemrev.2c00508}
}TY - JOUR AU - Rommens, Konstantijn T. AU - Saeys, Mark TI - Molecular Views on Fischer–Tropsch Synthesis JO - Chemical Reviews VL - 123 IS - 9 SP - 5798 EP - 5858 PY - 2023 DA - 2023/03/10 DO - 10.1021/acs.chemrev.2c00508 UR - https://doi.org/10.1021/acs.chemrev.2c00508 ER -
Add Find Research to Claude or ChatGPT and ask in plain language. The assistant reads this record, finds the papers around it and cites only what it actually found:
Setup takes about a minute: add the connector, then start the free trial.
Record from OpenAlex; open-access location from Unpaywall and the indexes. Find Research links only to legal copies.