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Yonggui Zhao, Devi Prasad Adiyeri Saseendran, Chong Huang, Carlos A. Triana, Walker R. Marks, Hang Chen, Han Zhao, Greta Ricarda Patzke
The oxygen evolution reaction (OER) and oxygen reduction reaction (ORR) are core steps of various energy conversion and storage systems. However, their sluggish reaction kinetics, i.e., the demanding multielectron transfer processes, still render OER/ORR catalysts less efficient for practical applications. Moreover, the complexity of the catalyst–electrolyte interface makes a comprehensive understanding of the intrinsic OER/ORR mechanisms challenging. Fortunately, recent advances of in situ / operando characterization techniques have facilitated the kinetic monitoring of catalysts under reaction conditions. Here we provide selected highlights of recent in situ / operando mechanistic studies of OER/ORR catalysts with the main emphasis placed on heterogeneous systems (primarily discussing first-row transition metals which operate under basic conditions), followed by a brief outlook on molecular catalysts. Key sections in this review are focused on determination of the true active species, identification of the active sites, and monitoring of the reactive intermediates. For in-depth insights into the above factors, a short overview of the metrics for accurate characterizations of OER/ORR catalysts is provided. A combination of the obtained time-resolved reaction information and reliable activity data will then guide the rational design of new catalysts. Strategies such as optimizing the restructuring process as well as overcoming the adsorption-energy scaling relations will be discussed. Finally, pending current challenges and prospects toward the understanding and development of efficient heterogeneous catalysts and selected homogeneous catalysts are presented.
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Zhao, Y., Saseendran, D. P. A., Huang, C., Triana, C. A., Marks, W. R., Chen, H., Zhao, H., & Patzke, G. R. (2023). Oxygen Evolution/Reduction Reaction Catalysts: From In Situ Monitoring and Reaction Mechanisms to Rational Design. Chemical Reviews, 123(9), 6257–6358. https://doi.org/10.1021/acs.chemrev.2c00515
Zhao, Yonggui, et al. "Oxygen Evolution/Reduction Reaction Catalysts: From In Situ Monitoring and Reaction Mechanisms to Rational Design." Chemical Reviews, vol. 123, no. 9, 2023, pp. 6257–6358, https://doi.org/10.1021/acs.chemrev.2c00515.
Zhao, Yonggui, Devi Prasad Adiyeri Saseendran, Chong Huang, Carlos A. Triana, Walker R. Marks, Hang Chen, Han Zhao, and Greta Ricarda Patzke. "Oxygen Evolution/Reduction Reaction Catalysts: From In Situ Monitoring and Reaction Mechanisms to Rational Design." Chemical Reviews 123, no. 9 (2023): 6257–6358. https://doi.org/10.1021/acs.chemrev.2c00515.
Zhao Y., Saseendran D. P. A., Huang C. [и др.] Oxygen Evolution/Reduction Reaction Catalysts: From In Situ Monitoring and Reaction Mechanisms to Rational Design // Chemical Reviews. — 2023. — Vol. 123, № 9. — P. 6257–6358. — URL: https://doi.org/10.1021/acs.chemrev.2c00515
@article{zhao2023oxygen,
title = {{Oxygen Evolution/Reduction Reaction Catalysts: From In Situ Monitoring and Reaction Mechanisms to Rational Design}},
author = {Yonggui Zhao and Devi Prasad Adiyeri Saseendran and Chong Huang and Carlos A. Triana and Walker R. Marks and Hang Chen and Han Zhao and Greta Ricarda Patzke},
journal = {Chemical Reviews},
year = {2023},
volume = {123},
number = {9},
pages = {6257--6358},
doi = {10.1021/acs.chemrev.2c00515},
url = {https://doi.org/10.1021/acs.chemrev.2c00515}
}TY - JOUR AU - Zhao, Yonggui AU - Saseendran, Devi Prasad Adiyeri AU - Huang, Chong AU - Triana, Carlos A. AU - Marks, Walker R. AU - Chen, Hang AU - Zhao, Han AU - Patzke, Greta Ricarda TI - Oxygen Evolution/Reduction Reaction Catalysts: From In Situ Monitoring and Reaction Mechanisms to Rational Design JO - Chemical Reviews VL - 123 IS - 9 SP - 6257 EP - 6358 PY - 2023 DA - 2023/03/21 DO - 10.1021/acs.chemrev.2c00515 UR - https://doi.org/10.1021/acs.chemrev.2c00515 ER -
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