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Kunyu Wang, Jiaqi Zhang, Yu‐Chuan Hsu, Hengyu Kengsley Lin, Zongsu Han, Jiandong Pang, Zhentao Yang, Rong‐Ran Liang, Wei Shi, Hong-Cai “Joe” Zhou
Enzymatic catalysis has fueled considerable interest from chemists due to its high efficiency and selectivity. However, the structural complexity and vulnerability hamper the application potentials of enzymes. Driven by the practical demand for chemical conversion, there is a long-sought quest for bioinspired catalysts reproducing and even surpassing the functions of natural enzymes. As nanoporous materials with high surface areas and crystallinity, metal-organic frameworks (MOFs) represent an exquisite case of how natural enzymes and their active sites are integrated into porous solids, affording bioinspired heterogeneous catalysts with superior stability and customizable structures. In this review, we comprehensively summarize the advances of bioinspired MOFs for catalysis, discuss the design principle of various MOF-based catalysts, such as MOF-enzyme composites and MOFs embedded with active sites, and explore the utility of these catalysts in different reactions. The advantages of MOFs as enzyme mimetics are also highlighted, including confinement, templating effects, and functionality, in comparison with homogeneous supramolecular catalysts. A perspective is provided to discuss potential solutions addressing current challenges in MOF catalysis.
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Wang, K., Zhang, J., Hsu, Y., Lin, H. K., Han, Z., Pang, J., Yang, Z., Liang, R., Shi, W., & Zhou, H.-C. “. (2023). Bioinspired Framework Catalysts: From Enzyme Immobilization to Biomimetic Catalysis. Chemical Reviews, 123(9), 5347–5420. https://doi.org/10.1021/acs.chemrev.2c00879
Wang, Kunyu, et al. "Bioinspired Framework Catalysts: From Enzyme Immobilization to Biomimetic Catalysis." Chemical Reviews, vol. 123, no. 9, 2023, pp. 5347–5420, https://doi.org/10.1021/acs.chemrev.2c00879.
Wang, Kunyu, Jiaqi Zhang, Yu‐Chuan Hsu, Hengyu Kengsley Lin, Zongsu Han, Jiandong Pang, Zhentao Yang, Rong‐Ran Liang, Wei Shi, and Hong-Cai “Joe” Zhou. "Bioinspired Framework Catalysts: From Enzyme Immobilization to Biomimetic Catalysis." Chemical Reviews 123, no. 9 (2023): 5347–5420. https://doi.org/10.1021/acs.chemrev.2c00879.
Wang K., Zhang J., Hsu Y. [и др.] Bioinspired Framework Catalysts: From Enzyme Immobilization to Biomimetic Catalysis // Chemical Reviews. — 2023. — Vol. 123, № 9. — P. 5347–5420. — URL: https://doi.org/10.1021/acs.chemrev.2c00879
@article{wang2023bioinspired,
title = {{Bioinspired Framework Catalysts: From Enzyme Immobilization to Biomimetic Catalysis}},
author = {Kunyu Wang and Jiaqi Zhang and Yu‐Chuan Hsu and Hengyu Kengsley Lin and Zongsu Han and Jiandong Pang and Zhentao Yang and Rong‐Ran Liang and Wei Shi and Hong-Cai “Joe” Zhou},
journal = {Chemical Reviews},
year = {2023},
volume = {123},
number = {9},
pages = {5347--5420},
doi = {10.1021/acs.chemrev.2c00879},
url = {https://doi.org/10.1021/acs.chemrev.2c00879}
}TY - JOUR AU - Wang, Kunyu AU - Zhang, Jiaqi AU - Hsu, Yu‐Chuan AU - Lin, Hengyu Kengsley AU - Han, Zongsu AU - Pang, Jiandong AU - Yang, Zhentao AU - Liang, Rong‐Ran AU - Shi, Wei AU - Zhou, Hong-Cai “Joe” TI - Bioinspired Framework Catalysts: From Enzyme Immobilization to Biomimetic Catalysis JO - Chemical Reviews VL - 123 IS - 9 SP - 5347 EP - 5420 PY - 2023 DA - 2023/04/12 DO - 10.1021/acs.chemrev.2c00879 UR - https://doi.org/10.1021/acs.chemrev.2c00879 ER -
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