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G. Murali, Jeevan Kumar Reddy Modigunta, Young Ho Park, Jong‐Hoon Lee, Jishu Rawal, Seul‐Yi Lee, Insik In, Soo‐Jin Park
Photocatalytic water splitting, CO 2 reduction, and pollutant degradation have emerged as promising strategies to remedy the existing environmental and energy crises. However, grafting of expensive and less abundant noble-metal cocatalysts on photocatalyst materials is a mandatory practice to achieve enhanced photocatalytic performance owing to the ability of the cocatalysts to extract electrons efficiently from the photocatalyst and enable rapid/enhanced catalytic reaction. Hence, developing highly efficient, inexpensive, and noble-metal-free cocatalysts composed of earth-abundant elements is considered as a noteworthy step toward considering photocatalysis as a more economical strategy. Recently, MXenes (two-dimensional (2D) transition-metal carbides, nitrides, and carbonitrides) have shown huge potential as alternatives for noble-metal cocatalysts. MXenes have several excellent properties, including atomically thin 2D morphology, metallic electrical conductivity, hydrophilic surface, and high specific surface area. In addition, they exhibit Gibbs free energy of intermediate H atom adsorption as close to zero and less than that of a commercial Pt-based cocatalyst, a Fermi level position above the H 2 generation potential, and an excellent ability to capture and activate CO 2 molecules. Therefore, there is a growing interest in MXene-based photocatalyst materials for various photocatalytic events. In this review, we focus on the recent advances in the synthesis of MXenes with 2D and 0D morphologies, the stability of MXenes, and MXene-based photocatalysts for H 2 evolution, CO 2 reduction, and pollutant degradation. The existing challenges and the possible future directions to enhance the photocatalytic performance of MXene-based photocatalysts are also discussed.
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Murali, G., Modigunta, J. K. R., Park, Y. H., Lee, J., Rawal, J., Lee, S., In, I., & Park, S. (2022). A Review on MXene Synthesis, Stability, and Photocatalytic Applications. ACS Nano, 16(9), 13370–13429. https://doi.org/10.1021/acsnano.2c04750
Murali, G., et al. "A Review on MXene Synthesis, Stability, and Photocatalytic Applications." ACS Nano, vol. 16, no. 9, 2022, pp. 13370–13429, https://doi.org/10.1021/acsnano.2c04750.
Murali, G., Jeevan Kumar Reddy Modigunta, Young Ho Park, Jong‐Hoon Lee, Jishu Rawal, Seul‐Yi Lee, Insik In, and Soo‐Jin Park. "A Review on MXene Synthesis, Stability, and Photocatalytic Applications." ACS Nano 16, no. 9 (2022): 13370–13429. https://doi.org/10.1021/acsnano.2c04750.
Murali G., Modigunta J. K. R., Park Y. H. [и др.] A Review on MXene Synthesis, Stability, and Photocatalytic Applications // ACS Nano. — 2022. — Vol. 16, № 9. — P. 13370–13429. — URL: https://doi.org/10.1021/acsnano.2c04750
@article{murali2022review,
title = {{A Review on MXene Synthesis, Stability, and Photocatalytic Applications}},
author = {G. Murali and Jeevan Kumar Reddy Modigunta and Young Ho Park and Jong‐Hoon Lee and Jishu Rawal and Seul‐Yi Lee and Insik In and Soo‐Jin Park},
journal = {ACS Nano},
year = {2022},
volume = {16},
number = {9},
pages = {13370--13429},
doi = {10.1021/acsnano.2c04750},
url = {https://doi.org/10.1021/acsnano.2c04750}
}TY - JOUR AU - Murali, G. AU - Modigunta, Jeevan Kumar Reddy AU - Park, Young Ho AU - Lee, Jong‐Hoon AU - Rawal, Jishu AU - Lee, Seul‐Yi AU - In, Insik AU - Park, Soo‐Jin TI - A Review on MXene Synthesis, Stability, and Photocatalytic Applications JO - ACS Nano VL - 16 IS - 9 SP - 13370 EP - 13429 PY - 2022 DA - 2022/09/12 DO - 10.1021/acsnano.2c04750 UR - https://doi.org/10.1021/acsnano.2c04750 ER -
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