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Li‐Wei Chen, Yuchen Hao, Yu Guo, Qinghua Zhang, Jiani Li, Wenyan Gao, Lantian Ren, Xin Su, Linyu Hu, Nan Zhang and 6 more
Photocatalytic nitrogen fixation reaction can harvest the solar energy to convert the abundant but inert N 2 into NH 3 . Here, utilizing metal–organic framework (MOF) membranes as the ideal assembly of nanoreactors to disperse and confine gold nanoparticles (AuNPs), we realize the direct plasmonic photocatalytic nitrogen fixation under ambient conditions. Upon visible irradiation, the hot electrons generated on the AuNPs can be directly injected into the N 2 molecules adsorbed on Au surfaces. Such N 2 molecules can be additionally activated by the strong but evanescently localized surface plasmon resonance field, resulting in a supralinear intensity dependence of the ammonia evolution rate with much higher apparent quantum efficiency and lower apparent activation energy under stronger irradiation. Moreover, the gas-permeable Au@MOF membranes, consisting of numerous interconnected nanoreactors, can ensure the dispersity and stability of AuNPs, further facilitate the mass transfer of N 2 molecules and (hydrated) protons, and boost the plasmonic photocatalytic reactions at the designed gas–membrane–solution interface. As a result, an ammonia evolution rate of 18.9 mmol g Au –1 h –1 was achieved under visible light (>400 nm, 100 mW cm –2 ) with an apparent quantum efficiency of 1.54% at 520 nm.
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Chen, L., Hao, Y., Guo, Y., Zhang, Q., Li, J., Gao, W., Ren, L., Su, X., Hu, L., Zhang, N., Li, S., Feng, X., Gu, L., Zhang, Y., Yin, A., & Wang, B. (2021). Metal–Organic Framework Membranes Encapsulating Gold Nanoparticles for Direct Plasmonic Photocatalytic Nitrogen Fixation. Journal of the American Chemical Society, 143(15), 5727–5736. https://doi.org/10.1021/jacs.0c13342
Chen, Li‐Wei, et al. "Metal–Organic Framework Membranes Encapsulating Gold Nanoparticles for Direct Plasmonic Photocatalytic Nitrogen Fixation." Journal of the American Chemical Society, vol. 143, no. 15, 2021, pp. 5727–5736, https://doi.org/10.1021/jacs.0c13342.
Chen, Li‐Wei, Yuchen Hao, Yu Guo, Qinghua Zhang, Jiani Li, Wenyan Gao, Lantian Ren, et al. "Metal–Organic Framework Membranes Encapsulating Gold Nanoparticles for Direct Plasmonic Photocatalytic Nitrogen Fixation." Journal of the American Chemical Society 143, no. 15 (2021): 5727–5736. https://doi.org/10.1021/jacs.0c13342.
Chen L., Hao Y., Guo Y. [и др.] Metal–Organic Framework Membranes Encapsulating Gold Nanoparticles for Direct Plasmonic Photocatalytic Nitrogen Fixation // Journal of the American Chemical Society. — 2021. — Vol. 143, № 15. — P. 5727–5736. — URL: https://doi.org/10.1021/jacs.0c13342
@article{chen2021metalorganic,
title = {{Metal–Organic Framework Membranes Encapsulating Gold Nanoparticles for Direct Plasmonic Photocatalytic Nitrogen Fixation}},
author = {Li‐Wei Chen and Yuchen Hao and Yu Guo and Qinghua Zhang and Jiani Li and Wenyan Gao and Lantian Ren and Xin Su and Linyu Hu and Nan Zhang and Siwu Li and Xiao Feng and Lin Gu and Ya‐Wen Zhang and Anxiang Yin and Bo Wang},
journal = {Journal of the American Chemical Society},
year = {2021},
volume = {143},
number = {15},
pages = {5727--5736},
doi = {10.1021/jacs.0c13342},
url = {https://doi.org/10.1021/jacs.0c13342}
}TY - JOUR AU - Chen, Li‐Wei AU - Hao, Yuchen AU - Guo, Yu AU - Zhang, Qinghua AU - Li, Jiani AU - Gao, Wenyan AU - Ren, Lantian AU - Su, Xin AU - Hu, Linyu AU - Zhang, Nan AU - Li, Siwu AU - Feng, Xiao AU - Gu, Lin AU - Zhang, Ya‐Wen AU - Yin, Anxiang AU - Wang, Bo TI - Metal–Organic Framework Membranes Encapsulating Gold Nanoparticles for Direct Plasmonic Photocatalytic Nitrogen Fixation JO - Journal of the American Chemical Society VL - 143 IS - 15 SP - 5727 EP - 5736 PY - 2021 DA - 2021/04/13 DO - 10.1021/jacs.0c13342 UR - https://doi.org/10.1021/jacs.0c13342 ER -
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