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Jieqiong Shan, Chao Ye, Shuangming Chen, Tulai Sun, Yan Jiao, Lingmei Liu, Chongzhi Zhu, Li Song, Yu Han, Mietek Jaroniec and 3 more
Noble metals manifest themselves with unique electronic structures and irreplaceable activity toward a wide range of catalytic applications but are unfortunately restricted by limited choice of geometric structures spanning single atoms, clusters, nanoparticles, and bulk crystals. Herein, we propose how to overcome this limitation by integrating noble metal atoms into the lattice of transition metal oxides to create a new type of hybrid structure. This study shows that iridium single atoms can be accommodated into the cationic sites of cobalt spinel oxide with short-range order and an identical spatial correlation as the host lattice. The resultant Ir 0.06 Co 2.94 O 4 catalyst exhibits much higher electrocatalytic activity than the parent oxide by 2 orders of magnitude toward the challenging oxygen evolution reaction under acidic conditions. Because of the strong interaction between iridium and cobalt oxide support, the Ir 0.06 Co 2.94 O 4 catalyst shows significantly improved corrosion resistance under acidic conditions and oxidative potentials. This work eliminates the “close-packing” limitation of noble metals and offers promising opportunity to create analogues with desired topologies for various catalytic applications.
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Shan, J., Ye, C., Chen, S., Sun, T., Jiao, Y., Liu, L., Zhu, C., Song, L., Han, Y., Jaroniec, M., Zhu, Y., Zheng, Y., & Qiao, S. (2021). Short-Range Ordered Iridium Single Atoms Integrated into Cobalt Oxide Spinel Structure for Highly Efficient Electrocatalytic Water Oxidation. Journal of the American Chemical Society, 143(13), 5201–5211. https://doi.org/10.1021/jacs.1c01525
Shan, Jieqiong, et al. "Short-Range Ordered Iridium Single Atoms Integrated into Cobalt Oxide Spinel Structure for Highly Efficient Electrocatalytic Water Oxidation." Journal of the American Chemical Society, vol. 143, no. 13, 2021, pp. 5201–5211, https://doi.org/10.1021/jacs.1c01525.
Shan, Jieqiong, Chao Ye, Shuangming Chen, Tulai Sun, Yan Jiao, Lingmei Liu, Chongzhi Zhu, et al. "Short-Range Ordered Iridium Single Atoms Integrated into Cobalt Oxide Spinel Structure for Highly Efficient Electrocatalytic Water Oxidation." Journal of the American Chemical Society 143, no. 13 (2021): 5201–5211. https://doi.org/10.1021/jacs.1c01525.
Shan J., Ye C., Chen S. [и др.] Short-Range Ordered Iridium Single Atoms Integrated into Cobalt Oxide Spinel Structure for Highly Efficient Electrocatalytic Water Oxidation // Journal of the American Chemical Society. — 2021. — Vol. 143, № 13. — P. 5201–5211. — URL: https://doi.org/10.1021/jacs.1c01525
@article{shan2021shortrange,
title = {{Short-Range Ordered Iridium Single Atoms Integrated into Cobalt Oxide Spinel Structure for Highly Efficient Electrocatalytic Water Oxidation}},
author = {Jieqiong Shan and Chao Ye and Shuangming Chen and Tulai Sun and Yan Jiao and Lingmei Liu and Chongzhi Zhu and Li Song and Yu Han and Mietek Jaroniec and Yihan Zhu and Yao Zheng and Shi‐Zhang Qiao},
journal = {Journal of the American Chemical Society},
year = {2021},
volume = {143},
number = {13},
pages = {5201--5211},
doi = {10.1021/jacs.1c01525},
url = {https://doi.org/10.1021/jacs.1c01525}
}TY - JOUR AU - Shan, Jieqiong AU - Ye, Chao AU - Chen, Shuangming AU - Sun, Tulai AU - Jiao, Yan AU - Liu, Lingmei AU - Zhu, Chongzhi AU - Song, Li AU - Han, Yu AU - Jaroniec, Mietek AU - Zhu, Yihan AU - Zheng, Yao AU - Qiao, Shi‐Zhang TI - Short-Range Ordered Iridium Single Atoms Integrated into Cobalt Oxide Spinel Structure for Highly Efficient Electrocatalytic Water Oxidation JO - Journal of the American Chemical Society VL - 143 IS - 13 SP - 5201 EP - 5211 PY - 2021 DA - 2021/03/25 DO - 10.1021/jacs.1c01525 UR - https://doi.org/10.1021/jacs.1c01525 ER -
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