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Chen‐Xu Liu, Wenwen Zhang, Si‐Yong Yin, Qing Gu, Shu‐Li You
Transition-metal-catalyzed enantioselective C-H functionalization has become a powerful strategy for the formation of C-C or C-X bonds, enabling the highly asymmetric synthesis of a wide range of enantioenriched compounds. Atropisomers are widely found in natural products and pharmaceutically relevant molecules, and have also found applications as privileged frameworks for chiral ligands and catalysts. Thus, research into asymmetric routes for the synthesis of atropisomers has garnered great interest in recent years. In this regard, transition-metal-catalyzed enantioselective C-H functionalization has emerged as an atom-economic and efficient strategy toward their synthesis. In this Perspective, the approaches for the synthesis of atropisomers by transition-metal-catalyzed asymmetric C-H functionalization reactions are summarized. The main focus here is on asymmetric catalysis via Pd, Rh, and Ir complexes, which have been the most frequently utilized catalysts among reported enantioselective C-H functionalization reactions. Finally, we discuss limitations on available protocols and give an outlook on possible future avenues of research.
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Liu, C., Zhang, W., Yin, S., Gu, Q., & You, S. (2021). Synthesis of Atropisomers by Transition-Metal-Catalyzed Asymmetric C–H Functionalization Reactions. Journal of the American Chemical Society, 143(35), 14025–14040. https://doi.org/10.1021/jacs.1c07635
Liu, Chen‐Xu, et al. "Synthesis of Atropisomers by Transition-Metal-Catalyzed Asymmetric C–H Functionalization Reactions." Journal of the American Chemical Society, vol. 143, no. 35, 2021, pp. 14025–14040, https://doi.org/10.1021/jacs.1c07635.
Liu, Chen‐Xu, Wenwen Zhang, Si‐Yong Yin, Qing Gu, and Shu‐Li You. "Synthesis of Atropisomers by Transition-Metal-Catalyzed Asymmetric C–H Functionalization Reactions." Journal of the American Chemical Society 143, no. 35 (2021): 14025–14040. https://doi.org/10.1021/jacs.1c07635.
Liu C., Zhang W., Yin S. [и др.] Synthesis of Atropisomers by Transition-Metal-Catalyzed Asymmetric C–H Functionalization Reactions // Journal of the American Chemical Society. — 2021. — Vol. 143, № 35. — P. 14025–14040. — URL: https://doi.org/10.1021/jacs.1c07635
@article{liu2021synthesis,
title = {{Synthesis of Atropisomers by Transition-Metal-Catalyzed Asymmetric C–H Functionalization Reactions}},
author = {Chen‐Xu Liu and Wenwen Zhang and Si‐Yong Yin and Qing Gu and Shu‐Li You},
journal = {Journal of the American Chemical Society},
year = {2021},
volume = {143},
number = {35},
pages = {14025--14040},
doi = {10.1021/jacs.1c07635},
url = {https://doi.org/10.1021/jacs.1c07635}
}TY - JOUR AU - Liu, Chen‐Xu AU - Zhang, Wenwen AU - Yin, Si‐Yong AU - Gu, Qing AU - You, Shu‐Li TI - Synthesis of Atropisomers by Transition-Metal-Catalyzed Asymmetric C–H Functionalization Reactions JO - Journal of the American Chemical Society VL - 143 IS - 35 SP - 14025 EP - 14040 PY - 2021 DA - 2021/08/25 DO - 10.1021/jacs.1c07635 UR - https://doi.org/10.1021/jacs.1c07635 ER -
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