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Long Jiao, Juntong Zhu, Yan Zhang, Weijie Yang, Siyuan Zhou, Aowen Li, Chenfan Xie, Xusheng Zheng, Wu Zhou, Shu‐Hong Yu, Hai‐Long Jiang
Single-atom catalysts (SACs), featuring high atom utilization, have captured widespread interests in diverse applications. However, the single-atom sites in SACs are generally recognized as independent units and the interplay of adjacent sites is largely overlooked. Herein, by the direct pyrolysis of MOFs assembled with Fe and Ni-doped ZnO nanoparticles, a novel Fe 1 –Ni 1 –N–C catalyst, with neighboring Fe and Ni single-atom pairs decorated on nitrogen-doped carbon support, has been precisely constructed. Thanks to the synergism of neighboring Fe and Ni single-atom pairs, Fe 1 –Ni 1 –N–C presents significantly boosted performances for electrocatalytic reduction of CO 2, far surpassing Fe 1 –N–C and Ni 1 –N–C with separate Fe or Ni single atoms. Additionally, the Fe 1 –Ni 1 –N–C also exhibits superior performance with excellent CO selectivity and durability in Zn-CO 2 battery. Theoretical simulations reveal that, in Fe 1 –Ni 1 –N–C, single Fe atoms can be highly activated by adjacent single-atom Ni via non-bonding interaction, significantly facilitating the formation of COOH* intermediate and thereby accelerating the overall CO 2 reduction. This work supplies a general strategy to construct single-atom catalysts containing multiple metal species and reveals the vital importance of the communitive effect between adjacent single atoms toward improved catalysis.
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Jiao, L., Zhu, J., Zhang, Y., Yang, W., Zhou, S., Li, A., Xie, C., Zheng, X., Zhou, W., Yu, S., & Jiang, H. (2021). Non-Bonding Interaction of Neighboring Fe and Ni Single-Atom Pairs on MOF-Derived N-Doped Carbon for Enhanced CO2 Electroreduction. Journal of the American Chemical Society, 143(46), 19417–19424. https://doi.org/10.1021/jacs.1c08050
Jiao, Long, et al. "Non-Bonding Interaction of Neighboring Fe and Ni Single-Atom Pairs on MOF-Derived N-Doped Carbon for Enhanced CO2 Electroreduction." Journal of the American Chemical Society, vol. 143, no. 46, 2021, pp. 19417–19424, https://doi.org/10.1021/jacs.1c08050.
Jiao, Long, Juntong Zhu, Yan Zhang, Weijie Yang, Siyuan Zhou, Aowen Li, Chenfan Xie, et al. "Non-Bonding Interaction of Neighboring Fe and Ni Single-Atom Pairs on MOF-Derived N-Doped Carbon for Enhanced CO2 Electroreduction." Journal of the American Chemical Society 143, no. 46 (2021): 19417–19424. https://doi.org/10.1021/jacs.1c08050.
Jiao L., Zhu J., Zhang Y. [и др.] Non-Bonding Interaction of Neighboring Fe and Ni Single-Atom Pairs on MOF-Derived N-Doped Carbon for Enhanced CO2 Electroreduction // Journal of the American Chemical Society. — 2021. — Vol. 143, № 46. — P. 19417–19424. — URL: https://doi.org/10.1021/jacs.1c08050
@article{jiao2021nonbonding,
title = {{Non-Bonding Interaction of Neighboring Fe and Ni Single-Atom Pairs on MOF-Derived N-Doped Carbon for Enhanced CO2 Electroreduction}},
author = {Long Jiao and Juntong Zhu and Yan Zhang and Weijie Yang and Siyuan Zhou and Aowen Li and Chenfan Xie and Xusheng Zheng and Wu Zhou and Shu‐Hong Yu and Hai‐Long Jiang},
journal = {Journal of the American Chemical Society},
year = {2021},
volume = {143},
number = {46},
pages = {19417--19424},
doi = {10.1021/jacs.1c08050},
url = {https://doi.org/10.1021/jacs.1c08050}
}TY - JOUR AU - Jiao, Long AU - Zhu, Juntong AU - Zhang, Yan AU - Yang, Weijie AU - Zhou, Siyuan AU - Li, Aowen AU - Xie, Chenfan AU - Zheng, Xusheng AU - Zhou, Wu AU - Yu, Shu‐Hong AU - Jiang, Hai‐Long TI - Non-Bonding Interaction of Neighboring Fe and Ni Single-Atom Pairs on MOF-Derived N-Doped Carbon for Enhanced CO2 Electroreduction JO - Journal of the American Chemical Society VL - 143 IS - 46 SP - 19417 EP - 19424 PY - 2021 DA - 2021/11/15 DO - 10.1021/jacs.1c08050 UR - https://doi.org/10.1021/jacs.1c08050 ER -
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