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Byung Hee Ko, Bjorn Hasa, Haeun Shin, Yaran Zhao, Feng Jiao
Mitigating nitrogen oxide (NO x ) emissions is critical to tackle global warming and improve air quality. Conventional NO x abatement technologies for emission control suffer from a low efficiency at near ambient temperatures. Herein, we show an electrochemical pathway to reduce gaseous NO x that can be conducted at high reaction rates (400 mA cm –2 ) under ambient conditions. Various transition metals are evaluated for electrochemical reduction of NO and N 2 O to reveal the role of electrocatalyst in determining the product selectivity. Specifically, Cu is highly selective toward NH 3 formation with >80% Faradaic efficiency in NO electroreduction. Furthermore, the partial pressure study of NO electroreduction revealed that a high NO coverage facilitates the N–N coupling reaction. In acidic electrolytes, the formation of NH 3 is greatly favored, whereas the N 2 production is suppressed. Additional mechanistic studies were conducted by using flow electrochemical mass spectrometry to gain further insights into reaction pathways. This work provides a promising avenue toward abating gaseous NO x emissions at ambient conditions by using renewable electricity.
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Ko, B. H., Hasa, B., Shin, H., Zhao, Y., & Jiao, F. (2022). Electrochemical Reduction of Gaseous Nitrogen Oxides on Transition Metals at Ambient Conditions. Journal of the American Chemical Society, 144(3), 1258–1266. https://doi.org/10.1021/jacs.1c10535
Ko, Byung Hee, et al. "Electrochemical Reduction of Gaseous Nitrogen Oxides on Transition Metals at Ambient Conditions." Journal of the American Chemical Society, vol. 144, no. 3, 2022, pp. 1258–1266, https://doi.org/10.1021/jacs.1c10535.
Ko, Byung Hee, Bjorn Hasa, Haeun Shin, Yaran Zhao, and Feng Jiao. "Electrochemical Reduction of Gaseous Nitrogen Oxides on Transition Metals at Ambient Conditions." Journal of the American Chemical Society 144, no. 3 (2022): 1258–1266. https://doi.org/10.1021/jacs.1c10535.
Ko B. H., Hasa B., Shin H. [и др.] Electrochemical Reduction of Gaseous Nitrogen Oxides on Transition Metals at Ambient Conditions // Journal of the American Chemical Society. — 2022. — Vol. 144, № 3. — P. 1258–1266. — URL: https://doi.org/10.1021/jacs.1c10535
@article{ko2022electrochemical,
title = {{Electrochemical Reduction of Gaseous Nitrogen Oxides on Transition Metals at Ambient Conditions}},
author = {Byung Hee Ko and Bjorn Hasa and Haeun Shin and Yaran Zhao and Feng Jiao},
journal = {Journal of the American Chemical Society},
year = {2022},
volume = {144},
number = {3},
pages = {1258--1266},
doi = {10.1021/jacs.1c10535},
url = {https://doi.org/10.1021/jacs.1c10535}
}TY - JOUR AU - Ko, Byung Hee AU - Hasa, Bjorn AU - Shin, Haeun AU - Zhao, Yaran AU - Jiao, Feng TI - Electrochemical Reduction of Gaseous Nitrogen Oxides on Transition Metals at Ambient Conditions JO - Journal of the American Chemical Society VL - 144 IS - 3 SP - 1258 EP - 1266 PY - 2022 DA - 2022/01/11 DO - 10.1021/jacs.1c10535 UR - https://doi.org/10.1021/jacs.1c10535 ER -
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