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Kui Liu, Hongmei Li, Minghao Xie, Pengfei Wang, Zhaoyu Jin, Yuanting Liu, Min Zhou, Panpan Li, Guihua Yu
The electrochemical nitrate reduction reaction (NO 3 RR) holds promise for converting nitrogenous pollutants to valuable ammonia products. However, conventional electrocatalysis faces challenges in effectively driving the complex eight-electron and nine-proton transfer process of the NO 3 RR while also competing with the hydrogen evolution reaction. In this study, we present the thermally enhanced electrocatalysis of nitrate-to-ammonia conversion over nickel-modified copper oxide single-atom alloy oxide nanowires. The catalyst demonstrates improved ammonia production performance with a Faradaic efficiency of approximately 80% and a yield rate of 9.7 mg h –1 cm –2 at +0.1 V versus a reversible hydrogen electrode at elevated cell temperatures. In addition, this thermally enhanced electrocatalysis system displays impressive stability, interference resistance, and favorable energy consumption and greenhouse gas emissions for the simulated industrial wastewater treatment. Complementary in situ analyses confirm that the significantly superior relay of active hydrogen species formed at Ni sites facilitates the thermal-field-coupled electrocatalysis of Cu surface-adsorbed *NO x hydrogenation. Theoretical calculations further support the thermodynamic and kinetic feasibility of the relay catalysis mechanism for the NO 3 RR over the Ni 1 Cu model catalyst. This study introduces a conceptual thermal-electrochemistry approach for the synergistic regulation of complex catalytic processes, highlighting the potential of multifield-coupled catalysis to advance sustainable-energy-powered chemical synthesis technologies.
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Liu, K., Li, H., Xie, M., Wang, P., Jin, Z., Liu, Y., Zhou, M., Li, P., & Yu, G. (2024). Thermally Enhanced Relay Electrocatalysis of Nitrate-to-Ammonia Reduction over Single-Atom-Alloy Oxides. Journal of the American Chemical Society, 146(11), 7779–7790. https://doi.org/10.1021/jacs.4c00429
Liu, Kui, et al. "Thermally Enhanced Relay Electrocatalysis of Nitrate-to-Ammonia Reduction over Single-Atom-Alloy Oxides." Journal of the American Chemical Society, vol. 146, no. 11, 2024, pp. 7779–7790, https://doi.org/10.1021/jacs.4c00429.
Liu, Kui, Hongmei Li, Minghao Xie, Pengfei Wang, Zhaoyu Jin, Yuanting Liu, Min Zhou, Panpan Li, and Guihua Yu. "Thermally Enhanced Relay Electrocatalysis of Nitrate-to-Ammonia Reduction over Single-Atom-Alloy Oxides." Journal of the American Chemical Society 146, no. 11 (2024): 7779–7790. https://doi.org/10.1021/jacs.4c00429.
Liu K., Li H., Xie M. [и др.] Thermally Enhanced Relay Electrocatalysis of Nitrate-to-Ammonia Reduction over Single-Atom-Alloy Oxides // Journal of the American Chemical Society. — 2024. — Vol. 146, № 11. — P. 7779–7790. — URL: https://doi.org/10.1021/jacs.4c00429
@article{liu2024thermally,
title = {{Thermally Enhanced Relay Electrocatalysis of Nitrate-to-Ammonia Reduction over Single-Atom-Alloy Oxides}},
author = {Kui Liu and Hongmei Li and Minghao Xie and Pengfei Wang and Zhaoyu Jin and Yuanting Liu and Min Zhou and Panpan Li and Guihua Yu},
journal = {Journal of the American Chemical Society},
year = {2024},
volume = {146},
number = {11},
pages = {7779--7790},
doi = {10.1021/jacs.4c00429},
url = {https://doi.org/10.1021/jacs.4c00429}
}TY - JOUR AU - Liu, Kui AU - Li, Hongmei AU - Xie, Minghao AU - Wang, Pengfei AU - Jin, Zhaoyu AU - Liu, Yuanting AU - Zhou, Min AU - Li, Panpan AU - Yu, Guihua TI - Thermally Enhanced Relay Electrocatalysis of Nitrate-to-Ammonia Reduction over Single-Atom-Alloy Oxides JO - Journal of the American Chemical Society VL - 146 IS - 11 SP - 7779 EP - 7790 PY - 2024 DA - 2024/03/11 DO - 10.1021/jacs.4c00429 UR - https://doi.org/10.1021/jacs.4c00429 ER -
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