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Stefano Michele Bernasconi, Mathieu Daëron, Kristin Bergmann, Magali Bonifacie, Anna Nele Meckler, Hagit P. Affek, Noah T. Anderson, David Bajnai, Eugeni Barkan, Emily J. Beverly and 51 more
Increased use and improved methodology of carbonate clumped isotope thermometry has greatly enhanced our ability to interrogate a suite of Earth‐system processes. However, interlaboratory discrepancies in quantifying carbonate clumped isotope (Δ 47 ) measurements persist, and their specific sources remain unclear. To address interlaboratory differences, we first provide consensus values from the clumped isotope community for four carbonate standards relative to heated and equilibrated gases with 1,819 individual analyses from 10 laboratories. Then we analyzed the four carbonate standards along with three additional standards, spanning a broad range of δ 47 and Δ 47 values, for a total of 5,329 analyses on 25 individual mass spectrometers from 22 different laboratories. Treating three of the materials as known standards and the other four as unknowns, we find that the use of carbonate reference materials is a robust method for standardization that yields interlaboratory discrepancies entirely consistent with intralaboratory analytical uncertainties. Carbonate reference materials, along with measurement and data processing practices described herein, provide the carbonate clumped isotope community with a robust approach to achieve interlaboratory agreement as we continue to use and improve this powerful geochemical tool. We propose that carbonate clumped isotope data normalized to the carbonate reference materials described in this publication should be reported as Δ 47 (I‐CDES) values for Intercarb‐Carbon Dioxide Equilibrium Scale.
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Bernasconi, S. M., Daëron, M., Bergmann, K., Bonifacie, M., Meckler, A. N., Affek, H. P., Anderson, N. T., Bajnai, D., Barkan, E., Beverly, E. J., Blamart, D., Burgener, L., Calmels, D., Chaduteau, C., Clog, M., Davidheiser‐Kroll, B., Davies, A., Dux, F. W., Eiler, J. M., … Ziegler, M. (2021). InterCarb: A Community Effort to Improve Interlaboratory Standardization of the Carbonate Clumped Isotope Thermometer Using Carbonate Standards. Geochemistry Geophysics Geosystems, 22(5), e2020GC009588. https://doi.org/10.1029/2020gc009588
Bernasconi, Stefano Michele, et al. "InterCarb: A Community Effort to Improve Interlaboratory Standardization of the Carbonate Clumped Isotope Thermometer Using Carbonate Standards." Geochemistry Geophysics Geosystems, vol. 22, no. 5, 2021, pp. e2020GC009588, https://doi.org/10.1029/2020gc009588.
Bernasconi, Stefano Michele, Mathieu Daëron, Kristin Bergmann, Magali Bonifacie, Anna Nele Meckler, Hagit P. Affek, Noah T. Anderson, et al. "InterCarb: A Community Effort to Improve Interlaboratory Standardization of the Carbonate Clumped Isotope Thermometer Using Carbonate Standards." Geochemistry Geophysics Geosystems 22, no. 5 (2021): e2020GC009588. https://doi.org/10.1029/2020gc009588.
Bernasconi S. M., Daëron M., Bergmann K. [и др.] InterCarb: A Community Effort to Improve Interlaboratory Standardization of the Carbonate Clumped Isotope Thermometer Using Carbonate Standards // Geochemistry Geophysics Geosystems. — 2021. — Vol. 22, № 5. — P. e2020GC009588. — URL: https://doi.org/10.1029/2020gc009588
@article{bernasconi2021intercarb,
title = {{InterCarb: A Community Effort to Improve Interlaboratory Standardization of the Carbonate Clumped Isotope Thermometer Using Carbonate Standards}},
author = {Stefano Michele Bernasconi and Mathieu Daëron and Kristin Bergmann and Magali Bonifacie and Anna Nele Meckler and Hagit P. Affek and Noah T. Anderson and David Bajnai and Eugeni Barkan and Emily J. Beverly and Dominique Blamart and Landon Burgener and Damien Calmels and Carine Chaduteau and Matthieu Clog and Brett Davidheiser‐Kroll and Amelia Davies and Florian W. Dux and John M. Eiler and Ben M. Elliott and Anne C. Fetrow and Jens Fiebig and Samuel L. Goldberg and Michaël Hermoso and Katharine W. Huntington and Ethan G. Hyland and Miquela Ingalls and Madalina Jaggi and Cédric M. John and Adam B. Jost and Sarah A. Katz and Julia R. Kelson and Tobias Kluge and Ilja Kocken and Amzad Hussain Laskar and Thomas Jan Leutert and Mao‐Chang Liang and Jamie Lucarelli and Tyler Mackey and Xavier Mangenot and Niklas Meinicke and Sevasti Modestou and Inigo A. Müller and Sean T. Murray and Ashling Neary and N. R. Packard and Benjamin H. Passey and E. Pelletier and Sierra Petersen and Alison M. Piasecki and Andrew J. Schauer and Kathryn E. Snell and Peter Koenraad Swart and Aradhna Tripati and Deepshikha Upadhyay and Torsten Walter Vennemann and Ian Z. Winkelstern and Drake A. Yarian and Naohiro Yoshida and Naizhong Zhang and Martin Ziegler},
journal = {Geochemistry Geophysics Geosystems},
year = {2021},
volume = {22},
number = {5},
pages = {e2020GC009588},
doi = {10.1029/2020gc009588},
url = {https://doi.org/10.1029/2020gc009588}
}TY - JOUR AU - Bernasconi, Stefano Michele AU - Daëron, Mathieu AU - Bergmann, Kristin AU - Bonifacie, Magali AU - Meckler, Anna Nele AU - Affek, Hagit P. AU - Anderson, Noah T. AU - Bajnai, David AU - Barkan, Eugeni AU - Beverly, Emily J. AU - Blamart, Dominique AU - Burgener, Landon AU - Calmels, Damien AU - Chaduteau, Carine AU - Clog, Matthieu AU - Davidheiser‐Kroll, Brett AU - Davies, Amelia AU - Dux, Florian W. AU - Eiler, John M. AU - Elliott, Ben M. AU - Fetrow, Anne C. AU - Fiebig, Jens AU - Goldberg, Samuel L. AU - Hermoso, Michaël AU - Huntington, Katharine W. AU - Hyland, Ethan G. AU - Ingalls, Miquela AU - Jaggi, Madalina AU - John, Cédric M. AU - Jost, Adam B. AU - Katz, Sarah A. AU - Kelson, Julia R. AU - Kluge, Tobias AU - Kocken, Ilja AU - Laskar, Amzad Hussain AU - Leutert, Thomas Jan AU - Liang, Mao‐Chang AU - Lucarelli, Jamie AU - Mackey, Tyler AU - Mangenot, Xavier AU - Meinicke, Niklas AU - Modestou, Sevasti AU - Müller, Inigo A. AU - Murray, Sean T. AU - Neary, Ashling AU - Packard, N. R. AU - Passey, Benjamin H. AU - Pelletier, E. AU - Petersen, Sierra AU - Piasecki, Alison M. AU - Schauer, Andrew J. AU - Snell, Kathryn E. AU - Swart, Peter Koenraad AU - Tripati, Aradhna AU - Upadhyay, Deepshikha AU - Vennemann, Torsten Walter AU - Winkelstern, Ian Z. AU - Yarian, Drake A. AU - Yoshida, Naohiro AU - Zhang, Naizhong AU - Ziegler, Martin TI - InterCarb: A Community Effort to Improve Interlaboratory Standardization of the Carbonate Clumped Isotope Thermometer Using Carbonate Standards JO - Geochemistry Geophysics Geosystems VL - 22 IS - 5 SP - e2020GC009588 PY - 2021 DA - 2021/04/14 DO - 10.1029/2020gc009588 UR - https://doi.org/10.1029/2020gc009588 ER -
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