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Jianfang Li, Zhaoyang Li, Xiangmei Liu, Changyi Li, Yufeng Zheng, Kwk Yeung, Zhenduo Cui, Yanqin Liang, Shengli Zhu, Wenbin Hu and 4 more
In view of increasing drug resistance, ecofriendly photoelectrical materials are promising alternatives to antibiotics. Here we design an interfacial Schottky junction of Bi2S3/Ti3C2Tx resulting from the contact potential difference between Ti3C2Tx and Bi2S3. The different work functions induce the formation of a local electrophilic/nucleophilic region. The self-driven charge transfer across the interface increases the local electron density on Ti3C2Tx. The formed Schottky barrier inhibits the backflow of electrons and boosts the charge transfer and separation. The photocatalytic activity of Bi2S3/Ti3C2Tx intensively improved the amount of reactive oxygen species under 808 nm near-infrared radiation. They kill 99.86% of Staphylococcus aureus and 99.92% of Escherichia coli with the assistance of hyperthermia within 10 min. We propose the theory of interfacial engineering based on work function and accordingly design the ecofriendly photoresponsive Schottky junction using two kinds of components with different work functions to effectively eradicate bacterial infection.
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Li, J., Li, Z., Liu, X., Li, C., Zheng, Y., Yeung, K., Cui, Z., Liang, Y., Zhu, S., Hu, W., Qi, Y., Zhang, T., Wang, X., & Wu, S. (2021). Interfacial engineering of Bi2S3/Ti3C2Tx MXene based on work function for rapid photo-excited bacteria-killing. Nature Communications, 12(1), 1224. https://doi.org/10.1038/s41467-021-21435-6
Li, Jianfang, et al. "Interfacial engineering of Bi2S3/Ti3C2Tx MXene based on work function for rapid photo-excited bacteria-killing." Nature Communications, vol. 12, no. 1, 2021, pp. 1224, https://doi.org/10.1038/s41467-021-21435-6.
Li, Jianfang, Zhaoyang Li, Xiangmei Liu, Changyi Li, Yufeng Zheng, Kwk Yeung, Zhenduo Cui, et al. "Interfacial engineering of Bi2S3/Ti3C2Tx MXene based on work function for rapid photo-excited bacteria-killing." Nature Communications 12, no. 1 (2021): 1224. https://doi.org/10.1038/s41467-021-21435-6.
Li J., Li Z., Liu X. [и др.] Interfacial engineering of Bi2S3/Ti3C2Tx MXene based on work function for rapid photo-excited bacteria-killing // Nature Communications. — 2021. — Vol. 12, № 1. — P. 1224. — URL: https://doi.org/10.1038/s41467-021-21435-6
@article{li2021interfacial,
title = {{Interfacial engineering of Bi2S3/Ti3C2Tx MXene based on work function for rapid photo-excited bacteria-killing}},
author = {Jianfang Li and Zhaoyang Li and Xiangmei Liu and Changyi Li and Yufeng Zheng and Kwk Yeung and Zhenduo Cui and Yanqin Liang and Shengli Zhu and Wenbin Hu and Yajun Qi and Tianjin Zhang and Xianbao Wang and Shuilin Wu},
journal = {Nature Communications},
year = {2021},
volume = {12},
number = {1},
pages = {1224},
doi = {10.1038/s41467-021-21435-6},
url = {https://doi.org/10.1038/s41467-021-21435-6}
}TY - JOUR AU - Li, Jianfang AU - Li, Zhaoyang AU - Liu, Xiangmei AU - Li, Changyi AU - Zheng, Yufeng AU - Yeung, Kwk AU - Cui, Zhenduo AU - Liang, Yanqin AU - Zhu, Shengli AU - Hu, Wenbin AU - Qi, Yajun AU - Zhang, Tianjin AU - Wang, Xianbao AU - Wu, Shuilin TI - Interfacial engineering of Bi2S3/Ti3C2Tx MXene based on work function for rapid photo-excited bacteria-killing JO - Nature Communications VL - 12 IS - 1 SP - 1224 PY - 2021 DA - 2021/02/22 DO - 10.1038/s41467-021-21435-6 UR - https://doi.org/10.1038/s41467-021-21435-6 ER -
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