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Yi Shi, Zhirui Ma, Yi-Ying Xiao, Yunchao Yin, Wenmao Huang, Zhichao Huang, Yunzhe Zheng, Fang-Ya Mu, Rong Tan Huang, Guoyue Shi and 3 more
Tuning metal-support interaction has been considered as an effective approach to modulate the electronic structure and catalytic activity of supported metal catalysts. At the atomic level, the understanding of the structure-activity relationship still remains obscure in heterogeneous catalysis, such as the conversion of water (alkaline) or hydronium ions (acid) to hydrogen (hydrogen evolution reaction, HER). Here, we reveal that the fine control over the oxidation states of single-atom Pt catalysts through electronic metal-support interaction significantly modulates the catalytic activities in either acidic or alkaline HER. Combined with detailed spectroscopic and electrochemical characterizations, the structure-activity relationship is established by correlating the acidic/alkaline HER activity with the average oxidation state of single-atom Pt and the Pt-H/Pt-OH interaction. This study sheds light on the atomic-level mechanistic understanding of acidic and alkaline HER, and further provides guidelines for the rational design of high-performance single-atom catalysts.
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Shi, Y., Ma, Z., Xiao, Y.-Y., Yin, Y., Huang, W., Huang, Z., Zheng, Y., Mu, F.-Y., Huang, R. T., Shi, G., Sun, Y., Xia, X., & Chen, W. (2021). Electronic metal–support interaction modulates single-atom platinum catalysis for hydrogen evolution reaction. Nature Communications, 12(1), 3021. https://doi.org/10.1038/s41467-021-23306-6
Shi, Yi, et al. "Electronic metal–support interaction modulates single-atom platinum catalysis for hydrogen evolution reaction." Nature Communications, vol. 12, no. 1, 2021, pp. 3021, https://doi.org/10.1038/s41467-021-23306-6.
Shi, Yi, Zhirui Ma, Yi-Ying Xiao, Yunchao Yin, Wenmao Huang, Zhichao Huang, Yunzhe Zheng, et al. "Electronic metal–support interaction modulates single-atom platinum catalysis for hydrogen evolution reaction." Nature Communications 12, no. 1 (2021): 3021. https://doi.org/10.1038/s41467-021-23306-6.
Shi Y., Ma Z., Xiao Y.-Y. [и др.] Electronic metal–support interaction modulates single-atom platinum catalysis for hydrogen evolution reaction // Nature Communications. — 2021. — Vol. 12, № 1. — P. 3021. — URL: https://doi.org/10.1038/s41467-021-23306-6
@article{shi2021electronic,
title = {{Electronic metal–support interaction modulates single-atom platinum catalysis for hydrogen evolution reaction}},
author = {Yi Shi and Zhirui Ma and Yi-Ying Xiao and Yunchao Yin and Wenmao Huang and Zhichao Huang and Yunzhe Zheng and Fang-Ya Mu and Rong Tan Huang and Guoyue Shi and Yi‐Yang Sun and Xing‐Hua Xia and Wei Chen},
journal = {Nature Communications},
year = {2021},
volume = {12},
number = {1},
pages = {3021},
doi = {10.1038/s41467-021-23306-6},
url = {https://doi.org/10.1038/s41467-021-23306-6}
}TY - JOUR AU - Shi, Yi AU - Ma, Zhirui AU - Xiao, Yi-Ying AU - Yin, Yunchao AU - Huang, Wenmao AU - Huang, Zhichao AU - Zheng, Yunzhe AU - Mu, Fang-Ya AU - Huang, Rong Tan AU - Shi, Guoyue AU - Sun, Yi‐Yang AU - Xia, Xing‐Hua AU - Chen, Wei TI - Electronic metal–support interaction modulates single-atom platinum catalysis for hydrogen evolution reaction JO - Nature Communications VL - 12 IS - 1 SP - 3021 PY - 2021 DA - 2021/05/21 DO - 10.1038/s41467-021-23306-6 UR - https://doi.org/10.1038/s41467-021-23306-6 ER -
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