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Xuehua Wang, Xianghu Wang, Jianfeng Huang, Shaoxiang Li, Alan Meng, Zhenjiang Li
Construction of Z-scheme heterostructure is of momentous significance for realizing efficient photocatalytic water splitting. However, the consciously modulate of Z-scheme charge transfer is still a great challenge. Herein, interfacial Mo-S bond and internal electric field modulated Z-Scheme heterostructure composed by sulfur vacancies-rich ZnIn2S4 (Vs-ZIS) and MoSe2 was rationally fabricated for efficient photocatalytic hydrogen evolution. Systematic investigations reveal that Mo-S bond and internal electric field induce the Z-scheme charge transfer mechanism as confirmed by the SPS and DMPO spin-trapping EPR spectra. Under the intense synergy among the Mo-S bond, internal electric field and S-vacancies, the optimized photocatalyst exhibits ultrahigh hydrogen evolution rate of 63.21 mmol∙g-1·h-1 with an apparent quantum yield of 76.48% at 420 nm monochromatic light, which is about 18.8-fold of the pristine ZIS. This work affords a new inspiration on consciously modulating Z-scheme charge transfer by atomic-level interface control and internal electric field to signally promote the photocatalytic performance.
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Wang, X., Wang, X., Huang, J., Li, S., Meng, A., & Li, Z. (2021). Interfacial chemical bond and internal electric field modulated Z-scheme Sv-ZnIn2S4/MoSe2 photocatalyst for efficient hydrogen evolution. Nature Communications, 12(1), 4112. https://doi.org/10.1038/s41467-021-24511-z
Wang, Xuehua, et al. "Interfacial chemical bond and internal electric field modulated Z-scheme Sv-ZnIn2S4/MoSe2 photocatalyst for efficient hydrogen evolution." Nature Communications, vol. 12, no. 1, 2021, pp. 4112, https://doi.org/10.1038/s41467-021-24511-z.
Wang, Xuehua, Xianghu Wang, Jianfeng Huang, Shaoxiang Li, Alan Meng, and Zhenjiang Li. "Interfacial chemical bond and internal electric field modulated Z-scheme Sv-ZnIn2S4/MoSe2 photocatalyst for efficient hydrogen evolution." Nature Communications 12, no. 1 (2021): 4112. https://doi.org/10.1038/s41467-021-24511-z.
Wang X., Wang X., Huang J. [и др.] Interfacial chemical bond and internal electric field modulated Z-scheme Sv-ZnIn2S4/MoSe2 photocatalyst for efficient hydrogen evolution // Nature Communications. — 2021. — Vol. 12, № 1. — P. 4112. — URL: https://doi.org/10.1038/s41467-021-24511-z
@article{wang2021interfacial,
title = {{Interfacial chemical bond and internal electric field modulated Z-scheme Sv-ZnIn2S4/MoSe2 photocatalyst for efficient hydrogen evolution}},
author = {Xuehua Wang and Xianghu Wang and Jianfeng Huang and Shaoxiang Li and Alan Meng and Zhenjiang Li},
journal = {Nature Communications},
year = {2021},
volume = {12},
number = {1},
pages = {4112},
doi = {10.1038/s41467-021-24511-z},
url = {https://doi.org/10.1038/s41467-021-24511-z}
}TY - JOUR AU - Wang, Xuehua AU - Wang, Xianghu AU - Huang, Jianfeng AU - Li, Shaoxiang AU - Meng, Alan AU - Li, Zhenjiang TI - Interfacial chemical bond and internal electric field modulated Z-scheme Sv-ZnIn2S4/MoSe2 photocatalyst for efficient hydrogen evolution JO - Nature Communications VL - 12 IS - 1 SP - 4112 PY - 2021 DA - 2021/07/05 DO - 10.1038/s41467-021-24511-z UR - https://doi.org/10.1038/s41467-021-24511-z ER -
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