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Panlong Zhai, Mingyue Xia, Yunzhen Wu, Guanghui Zhang, Junfeng Gao, Bo Zhang, Shuyan Cao, Yan-ting Yann Zhang, Zhuwei Li, Zhaozhong Fan and 5 more
Rational design of single atom catalyst is critical for efficient sustainable energy conversion. However, the atomic-level control of active sites is essential for electrocatalytic materials in alkaline electrolyte. Moreover, well-defined surface structures lead to in-depth understanding of catalytic mechanisms. Herein, we report a single-atomic-site ruthenium stabilized on defective nickel-iron layered double hydroxide nanosheets (Ru 1 /D-NiFe LDH). Under precise regulation of local coordination environments of catalytically active sites and the existence of the defects, Ru 1 /D-NiFe LDH delivers an ultralow overpotential of 18 mV at 10 mA cm −2 for hydrogen evolution reaction, surpassing the commercial Pt/C catalyst. Density functional theory calculations reveal that Ru 1 /D-NiFe LDH optimizes the adsorption energies of intermediates for hydrogen evolution reaction and promotes the O–O coupling at a Ru–O active site for oxygen evolution reaction. The Ru 1 /D-NiFe LDH as an ideal model reveals superior water splitting performance with potential for the development of promising water-alkali electrocatalysts.
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Zhai, P., Xia, M., Wu, Y., Zhang, G., Gao, J., Zhang, B., Cao, S., Zhang, Y.-T. Y., Li, Z., Fan, Z., Wang, C., Zhang, X., Miller, J. T., Sun, L., & Hou, J. (2021). Engineering single-atomic ruthenium catalytic sites on defective nickel-iron layered double hydroxide for overall water splitting. Nature Communications, 12(1), 4587. https://doi.org/10.1038/s41467-021-24828-9
Zhai, Panlong, et al. "Engineering single-atomic ruthenium catalytic sites on defective nickel-iron layered double hydroxide for overall water splitting." Nature Communications, vol. 12, no. 1, 2021, pp. 4587, https://doi.org/10.1038/s41467-021-24828-9.
Zhai, Panlong, Mingyue Xia, Yunzhen Wu, Guanghui Zhang, Junfeng Gao, Bo Zhang, Shuyan Cao, et al. "Engineering single-atomic ruthenium catalytic sites on defective nickel-iron layered double hydroxide for overall water splitting." Nature Communications 12, no. 1 (2021): 4587. https://doi.org/10.1038/s41467-021-24828-9.
Zhai P., Xia M., Wu Y. [и др.] Engineering single-atomic ruthenium catalytic sites on defective nickel-iron layered double hydroxide for overall water splitting // Nature Communications. — 2021. — Vol. 12, № 1. — P. 4587. — URL: https://doi.org/10.1038/s41467-021-24828-9
@article{zhai2021engineering,
title = {{Engineering single-atomic ruthenium catalytic sites on defective nickel-iron layered double hydroxide for overall water splitting}},
author = {Panlong Zhai and Mingyue Xia and Yunzhen Wu and Guanghui Zhang and Junfeng Gao and Bo Zhang and Shuyan Cao and Yan-ting Yann Zhang and Zhuwei Li and Zhaozhong Fan and Chen Wang and Xiaomeng Zhang and Jeffrey T. Miller and Licheng Sun and Jungang Hou},
journal = {Nature Communications},
year = {2021},
volume = {12},
number = {1},
pages = {4587},
doi = {10.1038/s41467-021-24828-9},
url = {https://doi.org/10.1038/s41467-021-24828-9}
}TY - JOUR AU - Zhai, Panlong AU - Xia, Mingyue AU - Wu, Yunzhen AU - Zhang, Guanghui AU - Gao, Junfeng AU - Zhang, Bo AU - Cao, Shuyan AU - Zhang, Yan-ting Yann AU - Li, Zhuwei AU - Fan, Zhaozhong AU - Wang, Chen AU - Zhang, Xiaomeng AU - Miller, Jeffrey T. AU - Sun, Licheng AU - Hou, Jungang TI - Engineering single-atomic ruthenium catalytic sites on defective nickel-iron layered double hydroxide for overall water splitting JO - Nature Communications VL - 12 IS - 1 SP - 4587 PY - 2021 DA - 2021/07/28 DO - 10.1038/s41467-021-24828-9 UR - https://doi.org/10.1038/s41467-021-24828-9 ER -
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