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Yang Tang, Xinnan Mao, Ying Zhang, Xiaoping Wu, Lu Wang, Mingyu Chu, Chih‐Wen Pao, Shize Yang, Yong Xu, Xiaoqing Huang
CO 2 hydrogenation has attracted great attention, yet the quest for highly-efficient catalysts is driven by the current disadvantages of poor activity, low selectivity, and ambiguous structure-performance relationship. We demonstrate here that C 3 N 4 -supported Cu single atom catalysts with tailored coordination structures, namely, Cu–N 4 and Cu–N 3 , can serve as highly selective and active catalysts for CO 2 hydrogenation at low temperature. The modulation of the coordination structure of Cu single atom is readily realized by simply altering the treatment parameters. Further investigations reveal that Cu–N 4 favors CO 2 hydrogenation to form CH 3 OH via the formate pathway, while Cu–N 3 tends to catalyze CO 2 hydrogenation to produce CO via the reverse water-gas-shift (RWGS) pathway. Significantly, the CH 3 OH productivity and selectivity reach 4.2 mmol g –1 h –1 and 95.5%, respectively, for Cu–N 4 single atom catalyst. We anticipate this work will promote the fundamental researches on the structure-performance relationship of catalysts.
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Tang, Y., Mao, X., Zhang, Y., Wu, X., Wang, L., Chu, M., Pao, C., Yang, S., Xu, Y., & Huang, X. (2021). Coordination tailoring of Cu single sites on C3N4 realizes selective CO2 hydrogenation at low temperature. Nature Communications, 12(1), 6022. https://doi.org/10.1038/s41467-021-26316-6
Tang, Yang, et al. "Coordination tailoring of Cu single sites on C3N4 realizes selective CO2 hydrogenation at low temperature." Nature Communications, vol. 12, no. 1, 2021, pp. 6022, https://doi.org/10.1038/s41467-021-26316-6.
Tang, Yang, Xinnan Mao, Ying Zhang, Xiaoping Wu, Lu Wang, Mingyu Chu, Chih‐Wen Pao, Shize Yang, Yong Xu, and Xiaoqing Huang. "Coordination tailoring of Cu single sites on C3N4 realizes selective CO2 hydrogenation at low temperature." Nature Communications 12, no. 1 (2021): 6022. https://doi.org/10.1038/s41467-021-26316-6.
Tang Y., Mao X., Zhang Y. [и др.] Coordination tailoring of Cu single sites on C3N4 realizes selective CO2 hydrogenation at low temperature // Nature Communications. — 2021. — Vol. 12, № 1. — P. 6022. — URL: https://doi.org/10.1038/s41467-021-26316-6
@article{tang2021coordination,
title = {{Coordination tailoring of Cu single sites on C3N4 realizes selective CO2 hydrogenation at low temperature}},
author = {Yang Tang and Xinnan Mao and Ying Zhang and Xiaoping Wu and Lu Wang and Mingyu Chu and Chih‐Wen Pao and Shize Yang and Yong Xu and Xiaoqing Huang},
journal = {Nature Communications},
year = {2021},
volume = {12},
number = {1},
pages = {6022},
doi = {10.1038/s41467-021-26316-6},
url = {https://doi.org/10.1038/s41467-021-26316-6}
}TY - JOUR AU - Tang, Yang AU - Mao, Xinnan AU - Zhang, Ying AU - Wu, Xiaoping AU - Wang, Lu AU - Chu, Mingyu AU - Pao, Chih‐Wen AU - Yang, Shize AU - Xu, Yong AU - Huang, Xiaoqing TI - Coordination tailoring of Cu single sites on C3N4 realizes selective CO2 hydrogenation at low temperature JO - Nature Communications VL - 12 IS - 1 SP - 6022 PY - 2021 DA - 2021/10/15 DO - 10.1038/s41467-021-26316-6 UR - https://doi.org/10.1038/s41467-021-26316-6 ER -
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