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Jiace Hao, Zechao C. Zhuang, Kecheng Cao, Guohua Gao, Chan Wang, Feili Lai, Shuanglong Lu, Piming Ma, Weifu Dong, Tianxi X. Liu, Mingliang Du, Han Zhu
High-entropy alloys have received considerable attention in the field of catalysis due to their exceptional properties. However, few studies hitherto focus on the origin of their outstanding performance and the accurate identification of active centers. Herein, we report a conceptual and experimental approach to overcome the limitations of single-element catalysts by designing a FeCoNiXRu (X: Cu, Cr, and Mn) High-entropy alloys system with various active sites that have different adsorption capacities for multiple intermediates. The electronegativity differences between mixed elements in HEA induce significant charge redistribution and create highly active Co and Ru sites with optimized energy barriers for simultaneously stabilizing OH* and H* intermediates, which greatly enhances the efficiency of water dissociation in alkaline conditions. This work provides an in-depth understanding of the interactions between specific active sites and intermediates, which opens up a fascinating direction for breaking scaling relation issues for multistep reactions.
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Hao, J., Zhuang, Z. C., Cao, K., Gao, G., Wang, C., Lai, F., Lu, S., Ma, P., Dong, W., Liu, T. X., Du, M., & Zhu, H. (2022). Unraveling the electronegativity-dominated intermediate adsorption on high-entropy alloy electrocatalysts. Nature Communications, 13(1), 2662. https://doi.org/10.1038/s41467-022-30379-4
Hao, Jiace, et al. "Unraveling the electronegativity-dominated intermediate adsorption on high-entropy alloy electrocatalysts." Nature Communications, vol. 13, no. 1, 2022, pp. 2662, https://doi.org/10.1038/s41467-022-30379-4.
Hao, Jiace, Zechao C. Zhuang, Kecheng Cao, Guohua Gao, Chan Wang, Feili Lai, Shuanglong Lu, et al. "Unraveling the electronegativity-dominated intermediate adsorption on high-entropy alloy electrocatalysts." Nature Communications 13, no. 1 (2022): 2662. https://doi.org/10.1038/s41467-022-30379-4.
Hao J., Zhuang Z. C., Cao K. [и др.] Unraveling the electronegativity-dominated intermediate adsorption on high-entropy alloy electrocatalysts // Nature Communications. — 2022. — Vol. 13, № 1. — P. 2662. — URL: https://doi.org/10.1038/s41467-022-30379-4
@article{hao2022unraveling,
title = {{Unraveling the electronegativity-dominated intermediate adsorption on high-entropy alloy electrocatalysts}},
author = {Jiace Hao and Zechao C. Zhuang and Kecheng Cao and Guohua Gao and Chan Wang and Feili Lai and Shuanglong Lu and Piming Ma and Weifu Dong and Tianxi X. Liu and Mingliang Du and Han Zhu},
journal = {Nature Communications},
year = {2022},
volume = {13},
number = {1},
pages = {2662},
doi = {10.1038/s41467-022-30379-4},
url = {https://doi.org/10.1038/s41467-022-30379-4}
}TY - JOUR AU - Hao, Jiace AU - Zhuang, Zechao C. AU - Cao, Kecheng AU - Gao, Guohua AU - Wang, Chan AU - Lai, Feili AU - Lu, Shuanglong AU - Ma, Piming AU - Dong, Weifu AU - Liu, Tianxi X. AU - Du, Mingliang AU - Zhu, Han TI - Unraveling the electronegativity-dominated intermediate adsorption on high-entropy alloy electrocatalysts JO - Nature Communications VL - 13 IS - 1 SP - 2662 PY - 2022 DA - 2022/05/13 DO - 10.1038/s41467-022-30379-4 UR - https://doi.org/10.1038/s41467-022-30379-4 ER -
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