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Pengtang Wang, Hao Yang, Cheng Tang, Yu Shiang Wu, Yao Zheng, Tao Cheng, Kenneth R. Davey, Xiaoqing Huang, Shi‐Zhang Qiao
Electroreduction of carbon dioxide (CO 2 ) into multicarbon products provides possibility of large-scale chemicals production and is therefore of significant research and commercial interest. However, the production efficiency for ethanol (EtOH), a significant chemical feedstock, is impractically low because of limited selectivity, especially under high current operation. Here we report a new silver–modified copper–oxide catalyst (dCu 2 O/Ag 2.3% ) that exhibits a significant Faradaic efficiency of 40.8% and energy efficiency of 22.3% for boosted EtOH production. Importantly, it achieves CO 2 –to–ethanol conversion under high current operation with partial current density of 326.4 mA cm −2 at −0.87 V vs reversible hydrogen electrode to rank highly significantly amongst reported Cu–based catalysts. Based on in situ spectra studies we show that significantly boosted production results from tailored introduction of Ag to optimize the coordinated number and oxide state of surface Cu sites, in which the * CO adsorption is steered as both atop and bridge configuration to trigger asymmetric C–C coupling for stablization of EtOH intermediates.
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Wang, P., Yang, H., Tang, C., Wu, Y. S., Zheng, Y., Cheng, T., Davey, K. R., Huang, X., & Qiao, S. (2022). Boosting electrocatalytic CO2–to–ethanol production via asymmetric C–C coupling. Nature Communications, 13(1), 3754. https://doi.org/10.1038/s41467-022-31427-9
Wang, Pengtang, et al. "Boosting electrocatalytic CO2–to–ethanol production via asymmetric C–C coupling." Nature Communications, vol. 13, no. 1, 2022, pp. 3754, https://doi.org/10.1038/s41467-022-31427-9.
Wang, Pengtang, Hao Yang, Cheng Tang, Yu Shiang Wu, Yao Zheng, Tao Cheng, Kenneth R. Davey, Xiaoqing Huang, and Shi‐Zhang Qiao. "Boosting electrocatalytic CO2–to–ethanol production via asymmetric C–C coupling." Nature Communications 13, no. 1 (2022): 3754. https://doi.org/10.1038/s41467-022-31427-9.
Wang P., Yang H., Tang C. [и др.] Boosting electrocatalytic CO2–to–ethanol production via asymmetric C–C coupling // Nature Communications. — 2022. — Vol. 13, № 1. — P. 3754. — URL: https://doi.org/10.1038/s41467-022-31427-9
@article{wang2022boosting,
title = {{Boosting electrocatalytic CO2–to–ethanol production via asymmetric C–C coupling}},
author = {Pengtang Wang and Hao Yang and Cheng Tang and Yu Shiang Wu and Yao Zheng and Tao Cheng and Kenneth R. Davey and Xiaoqing Huang and Shi‐Zhang Qiao},
journal = {Nature Communications},
year = {2022},
volume = {13},
number = {1},
pages = {3754},
doi = {10.1038/s41467-022-31427-9},
url = {https://doi.org/10.1038/s41467-022-31427-9}
}TY - JOUR AU - Wang, Pengtang AU - Yang, Hao AU - Tang, Cheng AU - Wu, Yu Shiang AU - Zheng, Yao AU - Cheng, Tao AU - Davey, Kenneth R. AU - Huang, Xiaoqing AU - Qiao, Shi‐Zhang TI - Boosting electrocatalytic CO2–to–ethanol production via asymmetric C–C coupling JO - Nature Communications VL - 13 IS - 1 SP - 3754 PY - 2022 DA - 2022/06/29 DO - 10.1038/s41467-022-31427-9 UR - https://doi.org/10.1038/s41467-022-31427-9 ER -
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