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Jiadong Chen, Chunhong Chen, Minkai Qin, Ben Li, Binbin Lin, Qing Mao, Hongbin Yang, Bin Liu, Yong Wang
Noble metal electrocatalysts (e.g., Pt, Ru, etc.) suffer from sluggish kinetics of water dissociation for the electrochemical reduction of water to molecular hydrogen in alkaline and neutral pH environments. Herein, we found that an integration of Ru nanoparticles (NPs) on oxygen-deficient WO 3-x manifested a 24.0-fold increase in hydrogen evolution reaction (HER) activity compared with commercial Ru/C electrocatalyst in neutral electrolyte. Oxygen-deficient WO 3-x is shown to possess large capacity for storing protons, which could be transferred to the Ru NPs under cathodic potential. This significantly increases the hydrogen coverage on the surface of Ru NPs in HER and thus changes the rate-determining step of HER on Ru from water dissociation to hydrogen recombination.
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Chen, J., Chen, C., Qin, M., Li, B., Lin, B., Mao, Q., Yang, H., Liu, B., & Wang, Y. (2022). Reversible hydrogen spillover in Ru-WO3-x enhances hydrogen evolution activity in neutral pH water splitting. Nature Communications, 13(1), 5382. https://doi.org/10.1038/s41467-022-33007-3
Chen, Jiadong, et al. "Reversible hydrogen spillover in Ru-WO3-x enhances hydrogen evolution activity in neutral pH water splitting." Nature Communications, vol. 13, no. 1, 2022, pp. 5382, https://doi.org/10.1038/s41467-022-33007-3.
Chen, Jiadong, Chunhong Chen, Minkai Qin, Ben Li, Binbin Lin, Qing Mao, Hongbin Yang, Bin Liu, and Yong Wang. "Reversible hydrogen spillover in Ru-WO3-x enhances hydrogen evolution activity in neutral pH water splitting." Nature Communications 13, no. 1 (2022): 5382. https://doi.org/10.1038/s41467-022-33007-3.
Chen J., Chen C., Qin M. [и др.] Reversible hydrogen spillover in Ru-WO3-x enhances hydrogen evolution activity in neutral pH water splitting // Nature Communications. — 2022. — Vol. 13, № 1. — P. 5382. — URL: https://doi.org/10.1038/s41467-022-33007-3
@article{chen2022reversible,
title = {{Reversible hydrogen spillover in Ru-WO3-x enhances hydrogen evolution activity in neutral pH water splitting}},
author = {Jiadong Chen and Chunhong Chen and Minkai Qin and Ben Li and Binbin Lin and Qing Mao and Hongbin Yang and Bin Liu and Yong Wang},
journal = {Nature Communications},
year = {2022},
volume = {13},
number = {1},
pages = {5382},
doi = {10.1038/s41467-022-33007-3},
url = {https://doi.org/10.1038/s41467-022-33007-3}
}TY - JOUR AU - Chen, Jiadong AU - Chen, Chunhong AU - Qin, Minkai AU - Li, Ben AU - Lin, Binbin AU - Mao, Qing AU - Yang, Hongbin AU - Liu, Bin AU - Wang, Yong TI - Reversible hydrogen spillover in Ru-WO3-x enhances hydrogen evolution activity in neutral pH water splitting JO - Nature Communications VL - 13 IS - 1 SP - 5382 PY - 2022 DA - 2022/09/14 DO - 10.1038/s41467-022-33007-3 UR - https://doi.org/10.1038/s41467-022-33007-3 ER -
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