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Xiaoran Zhang, Xiaorong Zhu, Shuowen Bo, Chen Chen, Mengyi Qiu, Xiaoxiao Wei, Nihan He, Chao Ying Xie, Wei Chen, Jianyun Zheng and 5 more
Electrocatalytic urea synthesis emerged as the promising alternative of Haber–Bosch process and industrial urea synthetic protocol. Here, we report that a diatomic catalyst with bonded Fe–Ni pairs can significantly improve the efficiency of electrochemical urea synthesis. Compared with isolated diatomic and single-atom catalysts, the bonded Fe–Ni pairs act as the efficient sites for coordinated adsorption and activation of multiple reactants, enhancing the crucial C–N coupling thermodynamically and kinetically. The performance for urea synthesis up to an order of magnitude higher than those of single-atom and isolated diatomic electrocatalysts, a high urea yield rate of 20.2 mmol h −1 g −1 with corresponding Faradaic efficiency of 17.8% has been successfully achieved. A total Faradaic efficiency of about 100% for the formation of value-added urea, CO, and NH 3 was realized. This work presents an insight into synergistic catalysis towards sustainable urea synthesis via identifying and tailoring the atomic site configurations.
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Zhang, X., Zhu, X., Bo, S., Chen, C., Qiu, M., Wei, X., He, N., Xie, C. Y., Chen, W., Zheng, J., Chen, P., Jiang, S. P., Li, Y., Liu, Q., & Wang, S. (2022). Identifying and tailoring C–N coupling site for efficient urea synthesis over diatomic Fe–Ni catalyst. Nature Communications, 13(1), 5337. https://doi.org/10.1038/s41467-022-33066-6
Zhang, Xiaoran, et al. "Identifying and tailoring C–N coupling site for efficient urea synthesis over diatomic Fe–Ni catalyst." Nature Communications, vol. 13, no. 1, 2022, pp. 5337, https://doi.org/10.1038/s41467-022-33066-6.
Zhang, Xiaoran, Xiaorong Zhu, Shuowen Bo, Chen Chen, Mengyi Qiu, Xiaoxiao Wei, Nihan He, et al. "Identifying and tailoring C–N coupling site for efficient urea synthesis over diatomic Fe–Ni catalyst." Nature Communications 13, no. 1 (2022): 5337. https://doi.org/10.1038/s41467-022-33066-6.
Zhang X., Zhu X., Bo S. [и др.] Identifying and tailoring C–N coupling site for efficient urea synthesis over diatomic Fe–Ni catalyst // Nature Communications. — 2022. — Vol. 13, № 1. — P. 5337. — URL: https://doi.org/10.1038/s41467-022-33066-6
@article{zhang2022identifying,
title = {{Identifying and tailoring C–N coupling site for efficient urea synthesis over diatomic Fe–Ni catalyst}},
author = {Xiaoran Zhang and Xiaorong Zhu and Shuowen Bo and Chen Chen and Mengyi Qiu and Xiaoxiao Wei and Nihan He and Chao Ying Xie and Wei Chen and Jianyun Zheng and Pinsong Chen and San Ping Jiang and Yafei Li and Qinghua Liu and Shuangyin Wang},
journal = {Nature Communications},
year = {2022},
volume = {13},
number = {1},
pages = {5337},
doi = {10.1038/s41467-022-33066-6},
url = {https://doi.org/10.1038/s41467-022-33066-6}
}TY - JOUR AU - Zhang, Xiaoran AU - Zhu, Xiaorong AU - Bo, Shuowen AU - Chen, Chen AU - Qiu, Mengyi AU - Wei, Xiaoxiao AU - He, Nihan AU - Xie, Chao Ying AU - Chen, Wei AU - Zheng, Jianyun AU - Chen, Pinsong AU - Jiang, San Ping AU - Li, Yafei AU - Liu, Qinghua AU - Wang, Shuangyin TI - Identifying and tailoring C–N coupling site for efficient urea synthesis over diatomic Fe–Ni catalyst JO - Nature Communications VL - 13 IS - 1 SP - 5337 PY - 2022 DA - 2022/09/10 DO - 10.1038/s41467-022-33066-6 UR - https://doi.org/10.1038/s41467-022-33066-6 ER -
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