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Rong Zhang, Chuan Li, Huilin Cui, Yanbo Wang, Shaoce Zhang, Pei R. Li, Yue Hou, Ying Guo, Guojin Liang, Zhaodong Huang, Chao Peng, Chunyi Zhi
Most current research is devoted to electrochemical nitrate reduction reaction for ammonia synthesis under alkaline/neutral media while the investigation of nitrate reduction under acidic conditions is rarely reported. In this work, we demonstrate the potential of TiO 2 nanosheet with intrinsically poor hydrogen-evolution activity for selective and rapid nitrate reduction to ammonia under acidic conditions. Hybridized with iron phthalocyanine, the resulting catalyst displays remarkably improved efficiency toward ammonia formation owing to the enhanced nitrate adsorption, suppressed hydrogen evolution and lowered energy barrier for the rate-determining step. Then, an alkaline-acid hybrid Zn-nitrate battery was developed with high open-circuit voltage of 1.99 V and power density of 91.4 mW cm –2 . Further, the environmental sulfur recovery can be powered by above hybrid battery and the hydrazine-nitrate fuel cell can be developed for simultaneously hydrazine/nitrate conversion and electricity generation. This work demonstrates the attractive potential of acidic nitrate reduction for ammonia electrosynthesis and broadens the field of energy conversion.
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Zhang, R., Li, C., Cui, H., Wang, Y., Zhang, S., Li, P. R., Hou, Y., Guo, Y., Liang, G., Huang, Z., Peng, C., & Zhi, C. (2023). Electrochemical nitrate reduction in acid enables high-efficiency ammonia synthesis and high-voltage pollutes-based fuel cells. Nature Communications, 14(1), 8036. https://doi.org/10.1038/s41467-023-43897-6
Zhang, Rong, et al. "Electrochemical nitrate reduction in acid enables high-efficiency ammonia synthesis and high-voltage pollutes-based fuel cells." Nature Communications, vol. 14, no. 1, 2023, pp. 8036, https://doi.org/10.1038/s41467-023-43897-6.
Zhang, Rong, Chuan Li, Huilin Cui, Yanbo Wang, Shaoce Zhang, Pei R. Li, Yue Hou, et al. "Electrochemical nitrate reduction in acid enables high-efficiency ammonia synthesis and high-voltage pollutes-based fuel cells." Nature Communications 14, no. 1 (2023): 8036. https://doi.org/10.1038/s41467-023-43897-6.
Zhang R., Li C., Cui H. [и др.] Electrochemical nitrate reduction in acid enables high-efficiency ammonia synthesis and high-voltage pollutes-based fuel cells // Nature Communications. — 2023. — Vol. 14, № 1. — P. 8036. — URL: https://doi.org/10.1038/s41467-023-43897-6
@article{zhang2023electrochemical,
title = {{Electrochemical nitrate reduction in acid enables high-efficiency ammonia synthesis and high-voltage pollutes-based fuel cells}},
author = {Rong Zhang and Chuan Li and Huilin Cui and Yanbo Wang and Shaoce Zhang and Pei R. Li and Yue Hou and Ying Guo and Guojin Liang and Zhaodong Huang and Chao Peng and Chunyi Zhi},
journal = {Nature Communications},
year = {2023},
volume = {14},
number = {1},
pages = {8036},
doi = {10.1038/s41467-023-43897-6},
url = {https://doi.org/10.1038/s41467-023-43897-6}
}TY - JOUR AU - Zhang, Rong AU - Li, Chuan AU - Cui, Huilin AU - Wang, Yanbo AU - Zhang, Shaoce AU - Li, Pei R. AU - Hou, Yue AU - Guo, Ying AU - Liang, Guojin AU - Huang, Zhaodong AU - Peng, Chao AU - Zhi, Chunyi TI - Electrochemical nitrate reduction in acid enables high-efficiency ammonia synthesis and high-voltage pollutes-based fuel cells JO - Nature Communications VL - 14 IS - 1 SP - 8036 PY - 2023 DA - 2023/12/05 DO - 10.1038/s41467-023-43897-6 UR - https://doi.org/10.1038/s41467-023-43897-6 ER -
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