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Jacqueline Sophie Edge, Simon E. J. O’Kane, Ryan Prosser, Niall Kirkaldy, Anisha N. Patel, Alastair Hales, Abir Ghosh, Weilong Ai, Jingyi Chen, Yang Jiang and 10 more
The expansion of lithium-ion batteries from consumer electronics to larger-scale transport and energy storage applications has made understanding the many mechanisms responsible for battery degradation increasingly important. The literature in this complex topic has grown considerably; this perspective aims to distil current knowledge into a succinct form, as a reference and a guide to understanding battery degradation. Unlike other reviews, this work emphasises the coupling between the different mechanisms and the different physical and chemical approaches used to trigger, identify and monitor various mechanisms, as well as the various computational models that attempt to simulate these interactions. Degradation is separated into three levels: the actual mechanisms themselves, the observable consequences at cell level called modes and the operational effects such as capacity or power fade. Five principal and thirteen secondary mechanisms were found that are generally considered to be the cause of degradation during normal operation, which all give rise to five observable modes. A flowchart illustrates the different feedback loops that couple the various forms of degradation, whilst a table is presented to highlight the experimental conditions that are most likely to trigger specific degradation mechanisms. Together, they provide a powerful guide to designing experiments or models for investigating battery degradation.
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Edge, J. S., O’Kane, S. E. J., Prosser, R., Kirkaldy, N., Patel, A. N., Hales, A., Ghosh, A., Ai, W., Chen, J., Jiang, Y., Shen, L., Pang, M.-C., Diaz, L. B., Tomaszewska, A., Marzook, M. W., Radhakrishnan, K., Wang, H., Patel, Y., Wu, B., & Offer, G. J. (2021). Lithium ion battery degradation: what you need to know. Physical Chemistry Chemical Physics, 23(14), 8200–8221. https://doi.org/10.1039/d1cp00359c
Edge, Jacqueline Sophie, et al. "Lithium ion battery degradation: what you need to know." Physical Chemistry Chemical Physics, vol. 23, no. 14, 2021, pp. 8200–8221, https://doi.org/10.1039/d1cp00359c.
Edge, Jacqueline Sophie, Simon E. J. O’Kane, Ryan Prosser, Niall Kirkaldy, Anisha N. Patel, Alastair Hales, Abir Ghosh, et al. "Lithium ion battery degradation: what you need to know." Physical Chemistry Chemical Physics 23, no. 14 (2021): 8200–8221. https://doi.org/10.1039/d1cp00359c.
Edge J. S., O’Kane S. E. J., Prosser R. [и др.] Lithium ion battery degradation: what you need to know // Physical Chemistry Chemical Physics. — 2021. — Vol. 23, № 14. — P. 8200–8221. — URL: https://doi.org/10.1039/d1cp00359c
@article{edge2021lithium,
title = {{Lithium ion battery degradation: what you need to know}},
author = {Jacqueline Sophie Edge and Simon E. J. O’Kane and Ryan Prosser and Niall Kirkaldy and Anisha N. Patel and Alastair Hales and Abir Ghosh and Weilong Ai and Jingyi Chen and Yang Jiang and Li Shen and Mei-Chin Pang and Laura Bravo Diaz and Anna Tomaszewska and Mohamed Waseem Marzook and Karthik Radhakrishnan and Huizhi Wang and Yatish Patel and Billy Wu and Gregory James Offer},
journal = {Physical Chemistry Chemical Physics},
year = {2021},
volume = {23},
number = {14},
pages = {8200--8221},
doi = {10.1039/d1cp00359c},
url = {https://doi.org/10.1039/d1cp00359c}
}TY - JOUR AU - Edge, Jacqueline Sophie AU - O’Kane, Simon E. J. AU - Prosser, Ryan AU - Kirkaldy, Niall AU - Patel, Anisha N. AU - Hales, Alastair AU - Ghosh, Abir AU - Ai, Weilong AU - Chen, Jingyi AU - Jiang, Yang AU - Shen, Li AU - Pang, Mei-Chin AU - Diaz, Laura Bravo AU - Tomaszewska, Anna AU - Marzook, Mohamed Waseem AU - Radhakrishnan, Karthik AU - Wang, Huizhi AU - Patel, Yatish AU - Wu, Billy AU - Offer, Gregory James TI - Lithium ion battery degradation: what you need to know JO - Physical Chemistry Chemical Physics VL - 23 IS - 14 SP - 8200 EP - 8221 PY - 2021 DA - 2021/01/01 DO - 10.1039/d1cp00359c UR - https://doi.org/10.1039/d1cp00359c ER -
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